Publication

Accelerating Calculations of Ultrafast Time-Resolved Electronic Spectra with Efficient Quantum Dynamics Methods

Publications associées (32)

Automated all-functionals infrared and Raman spectra

Infrared and Raman spectroscopies are ubiquitous techniques employed in many experimental laboratories, thanks to their fast and non-destructive nature able to capture materials' features as spectroscopic fingerprints. Nevertheless, these measurements freq ...

Nature Portfolio2024

A Cavity-Microscope for Quantum Simulations with Locally-Controllable All-to-All Interactions

Nick Jacob Sauerwein

This thesis presents the development, construction, and benchmark of an experimental platform that combines cold fermionic 6Li atoms with locally controllable light-matter interactions. To enable local control, a new device, the cavity-microscope, was crea ...

EPFL2024

Pressure stabilization effect on the donor-acceptor polyiodide chains in tetraethylammonium bis(diiodine) triiodide - insights from Raman spectroscopy

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Polyiodides present high bonding flexibility already at ambient conditions, and undergo significant pressure-induced structural deformations. Resonant Raman spectroscopy has been widely used to study I-I bonds in various polyiodides, but it carries a risk ...

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Transition to chaos in extended systems and their quantum impurity models

Camille Didier Georges Aron

Chaos sets a fundamental limit to quantum-information processing schemes. We study the onset of chaos in spatially extended quantum many-body systems that are relevant to quantum optical devices. We consider an extended version of the Tavis-Cummings model ...

Iop Publishing Ltd2024

Large-cage occupation and quantum dynamics of hydrogen molecules in sII clathrate hydrates

Richard Gaal, Livia Eleonora Bove Kado, Umbertoluca Ranieri

Hydrogen clathrate hydrates are ice-like crystalline substances in which hydrogen molecules are trapped inside polyhedral cages formed by the water molecules. Small cages can host only a single H-2 molecule, while each large cage can be occupied by up to f ...

Aip Publishing2024

Nanomechanical resonators with low dissipation for quantum optomechanics

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Fields of technology as diverse as microwave filter construction, characterization of material interfaces with atomic precision, and detection of gravitational waves from astronomical sources employ mechanical resonators at their core. The utility of mecha ...

EPFL2023

Self-correcting quantum many-body control using reinforcement learning with tensor networks

Friederike Metz

Quantum many-body control is a central milestone en route to harnessing quantum technologies. However, the exponential growth of the Hilbert space dimension with the number of qubits makes it challenging to classically simulate quantum many-body systems an ...

NATURE PORTFOLIO2023

Public-Key Encryption with Quantum Keys

Khashayar Barooti

In the framework of Impagliazzo's five worlds, a distinction is often made between two worlds, one where public-key encryption exists (Cryptomania), and one in which only one-way functions exist (MiniCrypt). However, the boundaries between these worlds can ...

Springer International Publishing Ag2023

Security in the Presence of Quantum Adversaries

Khashayar Barooti

With the looming threat of large-scale quantum computers, a fair portion of recent cryptographic research has focused on examining cryptographic primitives from the perspective of a quantum adversary. Shor's 1994 result revealed that quantum computers can ...

EPFL2023

Surface-induced vibrational energy redistribution in methane/surface scattering depends on catalytic activity

Rainer Beck, Christopher Scott Reilly, Patrick Floss

Recent state-to-state experiments of methane scattering from Ni(111) and graphene-covered Ni(111) combined with quantum mechanical simulations suggest an intriguing correlation between the surface-induced vibrational energy redistribution (SIVR) during the ...

2023