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alpha-Diimine homologues of cisplatin: synthesis, speciation in DMSO/water and cytotoxicity

Paul Joseph Dyson, Lucinda Kate Batchelor, Silvia Schoch

The Pt(ii) -diimine complexes [PtCl2{N-2-(HCNR)(2)}] (R = C6H11, 1; 4-C6H10OH, 2; 4-C6H4CH3, 3; 4-C6H4OH, 4) and [PtCl2{N-2-(CH3CNOH)(2)}] (5) were prepared in 60-81% yields from the 1:1 molar reactions of cis-[PtCl2(DMSO)(2)] with the appropriate -diimine ...

ROYAL SOC CHEMISTRY2018

District heating and cooling energy network using CO2 as a heat and mass transfer fluid

François Maréchal, Daniel Favrat, Luc Girardin, Samuel Henchoz

The 5th generation compact district heating and cooling networks in a temperature range of 10 to 16 °C have a great potential for energy savings by providing a heat source for decentralized heating heat pumps, a cold source for air-conditioning and a heat ...

2018

Hydro-chemo-mechanical behavior of a sand/bentonite mixture upon wetting paths

Lyesse Laloui, Alessio Ferrari, Donatella Manca

Sand/bentonite (S/B) mixtures are considered as backfilling materials for nuclear waste storage. The paper presents an experimental campaign that was carried out to investigate the swelling behavior of a S/B mixture, under different hydro-chemo-mechanical ...

HKGES2018

Assessing the Effect of Calcite Impurities in Clay on Optimal Dehydroxylation Parameters for Enhanced Reactivity

Karen Scrivener, Franco Alberto Zunino Sommariva

This study focused on understanding the influence of different amounts of calcite impurities (0 to 10% by mass) on the optimal parameters for clay dehydroxylation and the reactivity of the final calcined clay. A surface response experimental design was use ...

SPRINGER2018

Over the last decades, a large understanding has been gained on the elastic properties of rocks. Rocks are, however, porous materials, which properties depend on both response of the bulk material and of the pores. Because in that case both the applied ext ...

Amer Geophysical Union2017

Kinetics of calcium sulfoaluminate with 1% iron oxide by isothermal and isoconversional methods

Yu Zhang, Xuerun Li

The influence of iron oxide (Fe2O3) on the formation and decomposition kinetics of calcium sulfoaluminate (C(4)A(3)$) formed from tricalcium aluminate and calcium sulfate was investigated by both isothermal and isoconversional methods. Rietveld quantitativ ...

Ice Publishing2017

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Compact district energy networks in a temperature range of 10 to 16°C have a great potential for energy savings by providing a heat source for decentralized heating heat pumps, a cold source for air-conditioning and a heat sink for refrigeration or cogener ...

2017

Partial Molar Volumes of Aqua Ions from First Principles

Alfredo Pasquarello, Julia Anna Wiktor

Partial molar volumes of ions in water solution are calculated through pressures obtained from ab initio molecular dynamics simulations. The correct definition of pressure in charged systems subject to periodic boundary conditions requires access to the va ...

Amer Chemical Soc2017

A 3-dimensional phase-field model is implemented to simulate the grain evolution in the final stage of liquid-phase sintering. The model considers a liquid phase and a polycrystalline solid phase. Results for varying ratios of the solid-solid interface ene ...

Elsevier Sci Ltd2017

Bentonite-based materials are studied as potential barriers for the geological disposal of radioactive waste. In this context, the hydro-mechanical behaviour of the engineered barrier is first characterized by free swelling conditions followed by constant ...

EDP Sciences2016