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We have performed an experimental investigation into the interaction of vacuum-ultraviolet synchrotron radiation with pyridine molecules in the gas phase. Specifically, a double-ion chamber spectrometer was used to measure the absolute photoabsorption cros ...
In this thesis, I present an experimental molecular beam surface scattering study of dynamical processes involved when HCl molecules are scattered from Au(111) and Ag(111) surfaces. I investigated vibrational excitation, translational inelasticity and diss ...
The present thesis work deals with the investigation of the heterogeneous reactions involving nitrate radical (NO3), dinitrogen pentoxide (N2O5) and ozone (O3) on surrogates of atmospheric mineral dust particles characteristic of the troposphere. An additi ...
The mechanisms leading to ionization of neutral gas by means of microwaves in the electron cyclotron range of frequencies in a simple toroidal plasma configuration are investigated in the TORPEX device (Fasoli A et al 2003 Bull. Am. Phys. Soc. 48 119). The ...
We report quantitative dissociation yields for the reaction CH3OH (v(OH))-->nhnu CH3+OH induced by infrared multiphoton excitation of methanol pre-excited to various levels of the OH stretching vibration (v(OH)=0, 1, 3, 5). The yields are measured by detec ...
Because the spectral d. of Rydberg states scales with the third power of the principal quantum no. n, the region immediately below at. and mol. ionization thresholds is spectrally very dense. Studying the properties of high at. and mol. Rydberg states just ...
The photoexcitation and photoionization dynamics of sodium atoms deposited on the surface of helium nanodroplets and aromatic molecules (aniline, phenol and toluene) embedded in the interior of droplets have been investigated by a variety of spectroscopic ...
Excitation spectra up to the ionization threshold are reported for barium atoms located on the surface of helium nanodroplets. For states with low principal quantum number, the resonances are substantially broadened and shifted towards higher energy with r ...
The ionization dynamics of He nanodroplets irradiated with intense femtosecond XUV pulses of up to 10^13 W/cm2 power density has been investigated by photoelectron spectroscopy. Helium droplets were resonantly excited to atomic-like 2p states with a photon ...
We report on the measurement of the instantaneous Kerr nonlinearity and the retarded alignment of air molecules CO2, N-2, and O-2 triggered by an intense, lambda-cubic terahertz pulse, a diffraction-and transform-limited single-cycle pulse. The strong-fiel ...