Concept

Artificial photosynthesis

Related publications (255)

IrOOH nanosheets as acid stable electrocatalysts for the oxygen evolution reaction

In solids, heterogeneous catalysis is inherently bound to reactions on the surface. Yet, atomically efficient preparation of specific surfaces and the characterization of their properties are impeding its applications towards a clean energy future. Here, w ...

2018

Hot Hole Collection and Photoelectrochemical CO2 Reduction with Plasmonic Au/p-GaN Photocathodes

Giulia Tagliabue

Harvesting nonequilibrium hot carriers from plasmonic-metal nanostructures offers unique opportunities for driving photochemical reactions at the nanoscale. Despite numerous examples of hot electron-driven processes, the realization of plasmonic systems ca ...

2018

Linking Morphology and Multi-Physical Transport in Structured Photoelectrodes

Sophia Haussener, Marco Cantoni, Silvan Suter, Yannick Kenneth Gaudy

Semiconductors with complex anisotropic morphologies in solar to chemical energy conversion devices enhance light absorption and overcome limiting charge transport in the solid. However, structuring the solid-liquid interface has also implications on conce ...

2018

Semiconducting van der Waals Interfaces as Artificial Semiconductors

Helmuth Berger, Evgeniy Ponomarev

Recent technical progress demonstrates the possibility of stacking together virtually any combination of atomically thin crystals of van der Waals bonded compounds to form new types of heterostructures and interfaces. As a result, there is the need to unde ...

2018

Organic Semiconductor Based Devices for Solar Water Splitting

Kevin Sivula, Liang Yao, Nestor Guijarro Carratala

Solution processable organic semiconductors are well-established as high-performance materials for inexpensive and scalable solar energy conversion in organic photovoltaic (OPV) devices, but their promise in the economic conversion of solar energy into che ...

2018

Photocatalytic Hydrogen Generation from a Visible-Light-Responsive Metal–Organic Framework System: Stability versus Activity of Molybdenum Sulfide Cocatalysts

Berend Smit, Andreas Züttel, Kyriakos Stylianou, Wen Luo, Daniele Ongari, Ngoc Tú Nguyên, Bardiya Valizadeh, Stavroula Kampouri, Ophélie Marie Planes

We report the use of two earth abundant molybdenum sulfide-based cocatalysts, Mo(3)S(13)(2-)clusters and 1T-MoS2 nanoparticles (NPs), in combination with the visible-light active metal-organic framework (MOF) MIL-125-NH2 for the photocatalytic generation o ...

2018

Resurgence of DSCs with copper electrolyte: a detailed investigation of interfacial charge dynamics with cobalt and iodine based electrolytes

Ulf Anders Hagfeldt

Deploying earth abundant copper as a redox mediator in dye-sensitized solar cells (DSCs) has been found to be a very promising strategy to achieve higher photovoltage and power conversion efficiencies in full sun (100 mW cm(-2)) and in low/diffuse light co ...

ROYAL SOC CHEMISTRY2018

Iron Oxide Photoelectrode with Multidimensional Architecture for Highly Efficient Photoelectrochemical Water Splitting

Jun Ho Yum

Nanostructured metal oxide semiconductors have shown outstanding performances in photoelectrochemical (PEC) water splitting, but limitations in light harvesting and charge collection have necessitated further advances in photo-electrode design. Herein, we ...

Wiley-V C H Verlag Gmbh2017

Defects on surface and interface for photoelectrochemical properties of hematite photoanodes

Yelin Hu

Hydrogen is a highly versatile fuel that may become one of the key solutions to face our future energy challenges. Among all these methods for hydrogen production, solar water splitting offers possible advantages regarding components integration, stability ...

EPFL2017

Heptacoordinate Co-II Complex: A New Architecture for Photochemical Hydrogen Production

Euro Solari, Albert Ruggi, Fiorella Lucarini, Serhii Vasylevskyi

The first heptacoordinate cobalt catalyst for light-driven hydrogen production in water has been synthesized and characterized. Photochemical experiments using Ru(bpy)(3) as photosensitizer gave a turnover number (TON) of 16300molH(2)(molcat.)(-1) ac ...

Wiley-V C H Verlag Gmbh2017

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