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Under certain conditions mass transfer limitations on the growth of cloud condensation nuclei (CCN) may have a significant impact on the number of droplets that can form in a cloud. The assumption that particles remain in equilibrium until activated may th ...
Models of aerosol scavenging and aqueous-phase oxidation of SO2 by H2O2 and O3 in a cloud updraft are compared. Bulk models considering only a single droplet size are compared with size-resolved models that explicitly simulate multiple aerosol and drop siz ...
Previous research on the direct effect of atmospheric aerosols on climate has estimated the average radiative forcing per unit sulfate mass, and has used this average to calculate the magnitude and spatial distribution of sulfate forcing. In this paper, we ...
Carbonyl sulfide (COS) was measured in polar firn air from one Arctic and two Antarctic locations. The air samples represent atmospheric composition from the early to mid-20th century up to the present day. This provides the longest record to date of atmos ...
In this work, we utilize a rich set of simulated and ground-based observational data in Tianjin, China to examine and compare the differences in aerosol acidity and composition predicted by three popular thermodynamic equilibrium models: ISORROPIA II, the ...
Meteorological conditions, gas-phase precursors, and aerosol acidity (pH) can influence the formation of secondary inorganic aerosols (SIA) in fine particulate matter (PM2.5). Most works related to the influence of pH and gas-phase precursors on SIA have b ...
A total of 16 global chemistry transport models and general circulation models have participated in this study; 14 models have been evaluated with regard to their ability to reproduce the near-surface observed number concentration of aerosol particles and ...
A Multicomponent Aerosol Dynamics Model (MADM) capable of solving the condensation/evaporation equation of atmospheric aerosols is presented. Condensable species may be organic and/or inorganic. For the inorganic constituents the equilibrium model ISORROPI ...
We systematically evaluate the relative influence of sources and sinks of particles in the remote marine boundary layer (MBL) to elucidate the principal factors that govern MBL aerosol behavior. Processes considered include: (1) surface flux of dimethyl su ...
