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Non-polar solvation dynamics has been investigated using steady-state absorption and emission spectroscopy of the NO A(2)Sigma(+)(3ssigma) Rydberg state in fluid Ar over a wide range of densities spanning the supercritical regime. Equilibrium molecular dyn ...
We address the problem of modeling received pulse trains in a multipath fading channel and of computing their exact spectrum. We propose a model based on point processes. Such model is very general, simple and tractable and it allows to account for various ...
The excitation of the Rydberg states is used to study the nonpolar solvation dynamics in supercrit. fluids (SCFs). The system NO in supercrit. Ar serves as the model system. First, the steady-state, absorption and fluorescence spectra of the NO X 2P-A 2S+( ...
The TCV tokamak is equipped with a four-channel ultrasoft x-ray monochromator allowing low resolution (lambda/Deltalambda similar to 30) measurements in the energy range 200-800eV. Its main purpose is to simultaneously monitor emission from four of the mai ...
The dynamics of electron bubble formation upon excitation of the A(3ss) Rydberg orbital of NO in solid Ne was studied by femtosecond pump-probe spectroscopy. The authors observe an ultrafast expansion of the bubble, followed by a vibrational recurrence in ...
The ultrafast dynamics of electronic bubble formation upon excitation of the A(3ss) Rydberg state of NO trapped in solid H2 and D2 was studied by femtosecond pump-probe spectroscopy. The evolution of the spherical bubble is followed in real time by a probe ...
This paper presents a general method for obtaining the exact power spectra of generic time hopping modulated signals. Based on a point process approach, it provides simpler proofs for existing results and a powerful rigorous and at the same time systematic ...
Mol.-dynamics simulations of structural relaxation in electronically excited NO-doped solid neon are presented. The NO impurity is excited to its lowest A (3ss) Rydberg state, inducing a rearrangement of the surrounding medium in the form of a bubble, due ...
The dynamics of electron bubble formation upon excitation of the A(3ss) Rydberg orbital of NO in solid Ne was studied by conventional spectroscopy and fs pump-probe spectroscopy. The fs pump pulse initiates the formation of a bubble by the expansion of the ...
The structural changes due to formation of electronic bubbles in solid D2 are studied by fluorescence, fluorescence-excitation, and fluorescence-depletion spectroscopy of the lowest Rydberg state, A 2S+(3ss), of the NO impurity. The A X band is strongly bl ...