Ultrafast laser spectroscopy

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Chemistry
Physical chemistry
Femtochemistry

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Formation Mechanism of Elemental Te Produced in Tellurite Glass Systems by Femtosecond Laser Irradiation

Yves Bellouard, Gözden Torun

The formation of elemental trigonal tellurium (t-Te) on tellurite glass surfaces exposed to femtosecond laser pulses is discussed. Specifically, the underlying elemental crystallization phenomenon is investigated by altering laser parameters in common tell ...

Wiley2023

Charge Dynamics Electron Microscopy Nanoscale Imaging of Femtosecond Plasma Dynamics

Fabrizio Carbone, Ivan Madan, Thomas La Grange, Giovanni Maria Vanacore, Gabriele Berruto, Ido Kaminer, Simone Gargiulo, Luca Piazza, Francesco Barantani, Tom Theodorus Antonius Lummen

Understanding and actively controlling the spatiotemporal dynamics of nonequilibrium electron clouds is fundamental for the design of light and electron sources, high power electronic devices, and plasma-based applications. However, electron clouds evolve ...

AMER CHEMICAL SOC2023

Femtosecond laser-induced modifications and self-organization in complex glass systems

Gözden Torun

Ultrashort laser pulses, i.e., pulses emitted shorter than a picosecond, can tailor material properties by introducing permanent modifications locally in three dimensions. Remarkably, under a certain exposure condition, these modifications are accompanied ...

EPFL2023

Targeted capillary photothrombosis via multiphoton excitation of Rose Bengal

Paul James Marchand

Microvascular stalling, the process occurring when a capillary temporarily loses perfusion, has gained increasing interest in recent years through its demonstrated presence in various neuropathologies. Studying the impact of such stalls on the surrounding ...

2023

Tunable pump compression and fast modulation for pulsed THz generation

Ileana-Cristina Benea-Chelmus, Alessandro Tomasino, Yazan Lampert Almahmoud, Shima Rajabali

We demonstrate tunable dispersion compensation of femtosecond pulses at telecom wavelengths for broadband Terahertz generation in 7.5-meter fiber link using a Silicon prism pair. The prism pair enhances the amplitude of the THz E-field in InGaAs photocondu ...

IEEE2023

GeSn as next-generation material for short-wave infrared single-photon detection

Andrea Giunto

In recent years, the automotive industry has aspired to bring self-driving vehicles to the general public and light detection and ranging (LiDAR) sensors have emerged as the preferred solution for car vision systems. At present, LiDAR technologies employ e ...

EPFL2023

On the interaction of femtosecond laser pulses with layered dielectric materials

Ruben Ricca

Materials properties are strictly dependent on their microstructure. The internal symmetries and the disposition of the constituting atoms of a material, which depend on its crystallographic structure, greatly affect its response to mechanical, electromagn ...

EPFL2023

Investigating the Effect of Crystal Morphology on Optoelectronic Properties of Zinc Phosphide Thin Films via Optical-pump Terahertz Probe Spectroscopy

Elias Zsolt Stutz, Jean-Baptiste Leran, Mahdi Zamani, Rajrupa Paul, Simon Robert Escobar Steinvall, Mirjana Dimitrievska, Léa Buswell

Zinc phosphide ( Zn3P2) is a promising earth-abundant material for solar cell applications but calls for the further understanding of its optoelectronic properties. In this work, we perform contact-free and noninvasive optical-pump terahertz probe (OPTP) s ...

IEEE2023

Ultrafast tunable lasers using lithium niobate integrated photonics

Tobias Kippenberg, Rui Ning Wang, Anat Siddharth, Mikhail Churaev, Viacheslav Snigirev, Junqiu Liu, Guanhao Huang

Early works(1) and recent advances in thin-film lithium niobate (LiNbO3) on insulator have enabled low-loss photonic integrated circuits(2,3), modulators with improved half-wave voltage(4,5), electro-optic frequency combs(6) and on-chip electro-optic devic ...

NATURE PORTFOLIO2023

Terahertz waveform synthesis in integrated thin-film lithium niobate platform

Ileana-Cristina Benea-Chelmus, Jérôme Faist, Francesca Fabiana Settembrini

Bridging the "terahertz gap" relies upon synthesizing arbitrary waveforms in the terahertz domain enabling applications that require both narrow band sources for sensing and few-cycle drives for classical and quantum objects. However, realization of custom ...

Nature Portfolio2023

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Investigating the Effect of Crystal Morphology on Optoelectronic Properties of Zinc Phosphide Thin Films via Optical-pump Terahertz Probe Spectroscopy

Elias Zsolt Stutz, Jean-Baptiste Leran, Mahdi Zamani, Rajrupa Paul, Simon Robert Escobar Steinvall, Mirjana Dimitrievska, Léa Buswell

IEEE2023