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This lecture covers the hydrogenation and dehydrogenation of pyridines and quinolines, focusing on the catalysts, reaction conditions, and mechanistic considerations. The instructor discusses the importance of these reactions in organometallic chemistry, pharmaceutical applications, and energy storage, emphasizing the need for efficient methods to access key compounds. Control experiments, catalytic cycles, and potential applications in various industries are explored, highlighting the significance of understanding reaction mechanisms and optimizing catalyst performance. The lecture also touches on the use of DFT studies to complement experimental findings and the challenges of scaling up reactions. Overall, the lecture provides insights into the complex interplay between catalyst design, reaction conditions, and practical applications in the field of organometallic chemistry.