Sophia Haussener

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Related publications (135)

Multiphysics model for assessing photoelectrochemical phenomena under concentrated irradiation

Sophia Haussener, Isaac Thomas Holmes-Gentle, Franky Esteban Bedoya Lora

A multiphysics model was developed for a photoelectrochemical (PEC) cell at the device level to simulate water splitting operating under concentrated irradiation (between 50 to 600 kW m−2). The 2D model couples charge, heat, mass, photon, and momentum tran ...

2023

Single emulsion drops for photocatalytic water splitting as a membrane-free approach to product separation

Sophia Haussener, Esther Amstad, Gaia De Angelis, Swarnava Nandy, Sangram Ashok Savant

The coevolution of hydrogen and oxygen during photocatalytic water splitting presents a challenge for efficient product separation. Here, we demonstrate membrane-free, drop-based photocatalytic water splitting with inherent product separation and competiti ...

2023

Kilowatt-scale solar hydrogen production system using a concentrated integrated photoelectrochemical device

Sophia Haussener, Saurabh Yuvraj Tembhurne, Clemens Gregor Suter, Isaac Thomas Holmes-Gentle

The production of synthetic fuels and chemicals from solar energy and abundant reagents offers a promising pathway to a sustainable fuel economy and chemical industry. For the production of hydrogen, photoelectrochemical or integrated photovoltaic and elec ...

2023

Pathways to enhance electrochemical CO2 reduction identified through direct pore-level modeling

Sophia Haussener, Etienne Boutin, Shuo Liu, Evan Fair Johnson

Electrochemical conversion of CO2 to fuels and valuable products is one pathway to reduce CO2 emissions. Electrolyzers using gas diffusion electrodes (GDEs) show much higher current densities than aqueous phase electrolyzers, yet models for multi-physical ...

2023

Assessment of the technological viability of photoelectrochemical devices for oxygen and fuel production on Moon and Mars

Sophia Haussener, Byron Stuart Ross

Human deep space exploration is presented with multiple challenges, such as the reliable, efficient and sustainable operation of life support systems. The production and recycling of oxygen, carbon dioxide (CO2) and fuels are hereby key, as a resource resu ...

Nature Research2023

Photovoltaics at multi-terawatt scale: Waiting is not an option

Sophia Haussener, Stefaan De Wolf

A major renewable-energy milestone occurred in 2022: Photovoltaics (PV) exceeded a global installed capacity of 1 TWdc. But despite considerable growth and cost reduction over time, PV is still a small part of global electricity generation (4 to 5% for 202 ...

American Association for the Advancement of Science2023

Recognizing the life and scientific contributions of a pioneer in solar thermochemistry: Prof. Aldo Steinfeld

Sophia Haussener

Professor Aldo Steinfeld's contributions to the fields of solar thermochemistry and energy conversion are extensive and impressive. His work has greatly contributed to the ongoing transition from fossil to renewable fuels. We, his former doctoral students ...

PERGAMON-ELSEVIER SCIENCE LTD2023

Design and operational guidelines of solar-driven catalytic conversion of CO2 and H2 to fuels

Sophia Haussener, Sha Li

Sunlight-powered catalytic conversion of CO2 and (green) H2 into fuels and chemicals via Sabatier and reverse water gas shift (RWGS) processes offers a promising solution to reduce greenhouse gas emissions and increase renewable energy utilization. The suc ...

ELSEVIER SCI LTD2023

Morphology and Transport Characterization of Catalyst Layers for CO2 Reduction

Sophia Haussener, Francesca Lorenzutti

Gas diffusion electrodes (GDEs) help to reduce transport limitations in devices for electrochemical CO2 reduction. Homogenized modeling of such devices requires input of morphological characteristics and effective transport properties of the porous structu ...

2023

Photoelectrochemical behaviour of photoanodes under high photon fluxes

Sophia Haussener, Isaac Thomas Holmes-Gentle, Franky Esteban Bedoya Lora, Lorenzo Aimone

The experimental behaviour of photoelectrochemical materials illuminated under high irradiance conditions >100 kW m−2 has not been studied despite being potentially advantageous for improving the photoelectrochemical performance and the system-level design ...

Royal Society of Chemistry2023

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Assessment of the technological viability of photoelectrochemical devices for oxygen and fuel production on Moon and Mars

Sophia Haussener, Byron Stuart Ross

Nature Research2023