Aparajita Singha

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Magnetic properties of surface-adsorbed single rare earth atoms, molecules, and atomic scale clusters

Aparajita Singha

This thesis presents combined experimental and theoretical investigations of nanoscale, surface-supported magnets based on rare earths (RE) to understand and control the magnetic properties down to the scale of single atoms. We present the effects of adato ...

EPFL2017

4 f occupancy and magnetism of rare-earth atoms adsorbed on metal substrates

Harald Brune, Stefano Rusponi, Jan Gui-Hyon Dreiser, Christian Wäckerlin, Pietro Gambardella, Fabio Donati, Aparajita Singha, Romana Baltic, Sebastian Stepanow

We report x-ray absorption spectroscopy and x-ray magnetic circular dichroism measurements as well as multiplet calculations for Dy, Ho, Er, and Tm atoms adsorbed on Pt(111), Cu(111), Ag(100), and Ag(111). In the gas phase, all four elements are divalent a ...

Amer Physical Soc2017

Magnetic Hysteresis in Er Trimers on Cu(111)

Harald Brune, Stefano Rusponi, Marina Pivetta, Jan Gui-Hyon Dreiser, Christian Wäckerlin, Fabio Donati, Aparajita Singha, Romana Baltic

We report magnetic hysteresis in Er clusters on. Cu(111) starting from the size-of three atoms. combining Xray magnetic circular dichroism, scanning tunneling microscopy, and mean-field nucleation theory, we determine the size dependent magnetic properties ...

American Chemical Society2016

Magnetic remanence in single atoms

Harald Brune, François Patthey, Stefano Rusponi, Christian Wäckerlin, Jan Gui-Hyon Dreiser, Pietro Gambardella, Fabio Donati, Zeljko Sljivancanin, Aparajita Singha, Romana Baltic

A permanent magnet retains a substantial fraction of its saturation magnetization in the absence of an external magnetic field. Realizing magnetic remanence in a single atom allows for storing and processing information in the smallest unit of matter. We s ...

American Association for the Advancement of Science2016

Single Molecule Activity Measurements of Cytochrome P450 Oxidoreductase Reveal the Existence of Two Discrete Functional States

Aparajita Singha, Dimitrios Stamou

Cell Press2015

Strong antiferromagnetic exchange between manganese phthalocyanine and ferromagnetic europium oxide

Stefano Rusponi, Christian Wäckerlin, Jan Gui-Hyon Dreiser, Fabio Donati, Aparajita Singha, Romana Baltic

We report on the antiferromagnetic exchange coupling between a submonolayer of Mn(II)-phthalocyanine molecules and a ferromagnetic Eu(II)-oxide thin film. The exchange energy is larger by nearly two orders of magnitude compared to previous studies involvin ...

Royal Society of Chemistry2015

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Single Molecule Activity Measurements of Cytochrome P450 Oxidoreductase Reveal the Existence of Two Discrete Functional States

Aparajita Singha, Dimitrios Stamou

Cell Press2015