Publications by Isaac Thomas Holmes-Gentle

Effect of Operating Conditions on the Degradation of BiVO4 Photoanodes

Sophia Haussener, Isaac Thomas Holmes-Gentle, Franky Esteban Bedoya Lora

This work investigates how irradiance, temperature, and electrolyte properties (pH, concentration, and flow rate), influence the degradation of spray-pyrolyzed BiVO4 photoanodes during water splitting for solar fuel production. A novel four-cell photoelect ...

Wiley2025

Optical characterization of a solar concentrating dish system

Sophia Haussener, Clemens Gregor Suter, Isaac Thomas Holmes-Gentle

Solar dishes concentrate the quasi-collimated sun light towards a focal point. Typically, the optical characterization consists of experimental flux map measurements and Monte-Carlo ray-tracing (MCRT) simulations, which are fitted based on experimental dat ...

Institute of Physics2024

High-throughput parallel testing of ten photoelectrochemical cells for water splitting: case study on the effects of temperature in hematite photoanodes

Sophia Haussener, Isaac Thomas Holmes-Gentle, Roberto Valenza, Franky Esteban Bedoya Lora

High-throughput testing of photoelectrochemical cells and materials under well-defined operating conditions can accelerate the discovery of new semiconducting materials, the characterization of the phenomena occurring at the semiconductor-electrolyte inter ...

Royal Soc Chemistry2024

Multiphysics model for assessing photoelectrochemical phenomena under concentrated irradiation

Sophia Haussener, Isaac Thomas Holmes-Gentle, Franky Esteban Bedoya Lora

A multiphysics model was developed for a photoelectrochemical (PEC) cell at the device level to simulate water splitting operating under concentrated irradiation (between 50 to 600 kW m−2). The 2D model couples charge, heat, mass, photon, and momentum tran ...

2023

Kilowatt-scale solar hydrogen production system using a concentrated integrated photoelectrochemical device

Sophia Haussener, Saurabh Yuvraj Tembhurne, Clemens Gregor Suter, Isaac Thomas Holmes-Gentle

The production of synthetic fuels and chemicals from solar energy and abundant reagents offers a promising pathway to a sustainable fuel economy and chemical industry. For the production of hydrogen, photoelectrochemical or integrated photovoltaic and elec ...

2023

Photoelectrochemical behaviour of photoanodes under high photon fluxes

Sophia Haussener, Isaac Thomas Holmes-Gentle, Franky Esteban Bedoya Lora, Lorenzo Aimone

The experimental behaviour of photoelectrochemical materials illuminated under high irradiance conditions >100 kW m−2 has not been studied despite being potentially advantageous for improving the photoelectrochemical performance and the system-level design ...

Royal Society of Chemistry2023

Dynamic system modeling of thermally-integrated concentrated PV-electrolysis

Sophia Haussener, Saurabh Yuvraj Tembhurne, Clemens Gregor Suter, Isaac Thomas Holmes-Gentle

Understanding the dynamic response of a solar fuel processing system utilizing concentrated solar radiation and made of a thermally-integrated photovoltaic (PV) and water electrolyzer (EC) is important for the design, development and implementation of this ...

2020