“Sandwich Reactor” for Heterogeneous Catalytic Processes: N2O Decomposition as a Case Study
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Rationalization and construction-aware design dominate the issue of realizability of freeform architecture. The former means the decomposition of an intended shape into parts which are sufficiently simple and efficient to manufacture; the latter refers to ...
Nitrous oxide is the third most important gas contributing to global warming and its concentration in the atmosphere is still on the rise. Nitric acid production represents the largest source of N2O in the chemical industry, with a total annual emission of ...
A stirred-tank reactor was built with the objective of rapid and accurate temperature control in the reaction vessel. A first-principles heat transfer model was developed for the jacketed batch system, with the jacket inlet temperature used to control the ...
Taylor & Francis2010
The use of zeolites for catalytic reactions is a field in continuous development. Since it was demonstrated that metal-zeolites are efficient catalysts for NOx abatement, decomposition of nitrous oxide (N2O) over Fe-containing zeolites has attracted great ...
EPFL2010
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We present applications of a recently developed method, the singular value decomposition inversion (SVD-I), for inverting line integrated multichannel interferometer measurements in fusion devices. The method expands the local electron density profiles int ...
2004
Al/SiC composites with volume fractions of SiC between 0.55 and 0.71 were made from identical tapped and vibrated powder preforms by squeeze casting (SC) and by two different setups for gas pressure infiltration (GPI), one that allows short (1-2 min) liqui ...
Springer US2010
The objective of this thesis is the development of a compact reactor for continuous three-phase reactions in single-pass configurations. The design is based on a bubble column reactor staged with layers of catalytic material. To make the reactor suitable f ...
EPFL2009
The reaction mechanism for nitrous oxide (N2O) direct decomposition into molecular nitrogen and oxygen was studied on binuclear iron sites in Fe-ZSM-5 zeolite using the density functional theory (DFT). Starting from the hydroxylated bi-iron complex ...
2008
This chapter contains sections titled: - Introduction - Stochastic Programming Concepts - A Capacity Expansion Model - Probabilistic Model - Decomposition Algorithms - Acknowledgements - References ...
Wiley-VCH2008
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This study aims at an investigation of the impurity gases emitted during the decomposition of borohydrides. For this we have set up a quantitative gas analysis based on a combination of FTIR spectroscopy and gravimetry. We show that the emission of various ...
