Ultraviolet-visible absorption of small silver clusters in neon: Ag-n (n=1-9)
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This thesis is devoted to the study of the optical properties of small metal clusters and metal cluster organic compounds. For this purpose a ultra-high vacuum (UHV) experimental apparatus has been built which allows for the deposition of mass selected neu ...
A detailed computational characterization of the one-photon absorption spectrum of a 2-((E)-2-[ 2,2']-bithiophenyl-5-yl-vinyl)-1-methyl-quinolinium cation in acetonitrile solution is presented. The main physico-chemical effects (solvation, vibronic progres ...
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Nature Publishing Group2017
The optical gap of the organic semiconductor [1]benzothieno[3,2-b]benzothiophene and its 2,7-dibrominated analogue is measured in solution and in the crystalline state by means of UV-vis and emission spectroscopy. Bromination leads to a change in molecular ...
Royal Soc Chemistry2014
Plasma wind tunnel experiments have been performed simulating a Hayabusa reentry trajectory point at 78.8km altitude with a velocity of 11.7km/s corresponding to a local mass-specific enthalpy of 68.4MJ/kg and a stagnation pressure of 2.44kPa. Ablation-rad ...
American Institute of Aeronautics and Astronautics2017
A wide variety of physicochemical processes at a molecular level, in particular charge or energy transfer, electronic and vibrational relaxation, are at the origin of biological functionality of proteins and organometallic compounds. The work reported in t ...
EPFL2015
It is known that excitation by visible light of the singlet metal-to-ligand charge-transfer (1MLCT) states of Fe(II) complexes leads to population of the lowest-lying high-spin quintet state (T-5) with unity quantum yield. Here we investigate this so-calle ...
Nature Publishing Group2015
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A green laser pointer shone through a glass of cola will appear red when looking from above the glass. Lowering the laser so that it is deeper in the cola, the colour will vary from orange to deep red. Fluorescence and absorption spectra were recorded cons ...
We introduce a new method to compute the optical absorption spectra of complex molecular systems in solution, based on the Liouville approach to time-dependent density-functional perturbation theory and the revised self-consistent continuum solvation model ...
One approach to reducing the bandgap is the utilization of ternary and quaternary oxides, which have been receiving increased attention as light absorbers that, critically, also supply the potential needed to drive multi-electron oxidn. reactions. In this ...
