A Vibronic Coupling Hamiltonian to Describe the Ultrafast Excited State Dynamics of a Cu(I)-Phenanthroline Complex
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Results of present and previous measurements of the23Na NMR response, dc- and ac-magnetic susceptibilities and the specific heat ofNa2V3O7at low temperatures suggest that this material is close to a quantum critical point (QCP) atm0H¼0 T. The experimental ...
Femtosecond fluorescence-upconversion studies of aq. [Ru(bpy)3]2+ show a short-lived vibrationally hot emission of the singlet metal-to-ligand charge-transfer state, with an ultrafast intersystem crossing (~ 10 fs) to the triplet state at const. energy (th ...
The formation and quenching of the triplet state of xanthone are studied by femtosecond techniques. As revealed by femtosecond fluorescence spectroscopy, the primarily excited 1ππ* state decays within 1.5 ps. In a transient absorption experiment, this time ...
The authors present a hybrid Car-Parrinello quantum mech./mol. mech. (QM/MM) approach that is capable of treating the dynamics of mol. systems in electronically excited states in complex environments. The potential energy surface in the excited state is de ...
