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Phase-resolved particle size distribution: New insight into material characterization

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The use of mixed-linker metal-organic frameworks (MIXMOFs) is one of the most effective strategies to modulate the physical-chemical properties of MOFs without affecting the overall crystal structure. In many instances, MIXMOFs have been recognized as soli ...

2017

Assessment of phase-field-crystal concepts using long-time molecular dynamics

William Curtin, Kristopher Learion Baker

The ability of the phase-field-crystal (PFC) model to quantitatively predict atomistic defect structures in crystalline solids is addressed. First, general aspects of the PFC model are discussed within the context of obtaining quantitative results in solid ...

American Physical Society2015

In situ X-ray Diffraction during Casting: Study of Hot Tearing in Al-Zn alloys

Jean-Marie Drezet, Güven Kurtuldu, Bastien Gilbert Pierre Mireux

During solidification of metallic alloys, coalescence corresponds to the formation of solid bridges between grains when both solid and liquid phases are percolated. As such, it represents a key transition with respect to the mechanical behaviour of solidif ...

Trans Tech Publications Switzerland2015

Criticality in the Approach to Failure in Amorphous Solids

Matthieu Wyart, Jie Lin

Failure of amorphous solids is fundamental to various phenomena, including landslides and earthquakes. Recent experiments indicate that highly plastic regions form elongated structures that are especially apparent near the maximal shear stress Sigma(max) w ...

American Physical Society2015

'Seeing' Atoms: The Crystallographic Revolution

Dieter Schwarzenbach

Laue's experiment in 1912 of the diffraction of X-rays by crystals led to one of the most influential discoveries in the history of science: the first determinations of crystal structures, NaCl and diamond in particular, by W. L. Bragg in 1913. For the fir ...

Swiss Chemical Soc2014

In situ Neutron Diffraction during Casting: Determination of Rigidity Point in Grain Refined Al-Cu Alloys

Jean-Marie Drezet, Bastien Gilbert Pierre Mireux

The rigidity temperature of a solidifying alloy is the temperature at which the solid plus liquid phases are sufficiently coalesced to transmit long range tensile strains and stresses. It determines the point at which thermally induced deformations start t ...

Mdpi Ag2014

Kinetically tuned dimensional augmentation as a versatile synthetic route towards robust metal-organic frameworks

Berend Smit, Cory Matthew Simon

Metal-organic frameworks with high stability have been pursued for many years due to the sustainability requirement for practical applications. However, researchers have had great difficulty synthesizing chemically ultra-stable, highly porous metal-organic ...

Nature Publishing Group2014

In recent years quantum antiferromagnets with an intrinsically disordered (“spin liquid”) ground state and an energy gap in the spin excitation spectrum have received a great deal of attention. In search for new experimental realizations of spin-ladder and ...

EPFL2013

Mapping of Functional Groups in Metal-Organic Frameworks

Berend Smit, Ji Hyun Kim

We determined the heterogeneous mesoscale spatial apportionment of functional groups in a series of multivariate metal-organic frameworks (MTV-MOF-5) containing BDC (1,4-benzenedicarboxylate) linkers with different functional groups - B (BDC-NH2), E (BDC-N ...

2013

Slurries are widely used in important chemical and pharmaceutical manufacturing processes. In this presentation we report chemical monitoring and modeling of batch slurry reactions using optical and calorimetric measurement where key analytes are present i ...

2012