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Measuring absolute spin polarization in dissolution-DNP by Spin PolarimetrY Magnetic Resonance (SPY-MR)

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The time-window for processing electron spin information (spintronics) in solid-state quantum electronic devices is determined by the spin-lattice and spin-spin relaxation times of electrons. Minimizing the effects of spin-orbit coupling and the local magn ...

Nature Publishing Group2016

Novel Instrumentation and Methods for Chemical Applications of Dissolution Dynamic Nuclear Polarization

Jonas Milani

One of the major disadvantages of Nuclear Magnetic Resonance (NMR) is its low sensitivity, mainly due to a very low spin polarization. Since 2003, Dissolution Dynamic Nuclear Polarization (D-DNP) provides a way of overcoming this drawback in solution by in ...

EPFL2016

Long-lived nuclear spin states of magnetically equivalent protons by means of dissolution dynamic nuclear polarization

Daniele Mammoli

Nuclear Magnetic Resonance (NMR) is one of the most versatile techniques since it enables the characterization of solid, liquid and gaseous systems in a plethora of in-vitro and in-vivo experiments. Despite its multidisciplinary scope, it still suffers fro ...

EPFL2016

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We report electron spin resonance (ESR) measurements on stage-I potassium intercalated graphite (KC8). Angular dependent measurements show that the spin-lattice relaxation time is longer when the magnetic field is perpendicular to the graphene layer as com ...

Wiley-V C H Verlag Gmbh2016

Transportable long-lived hyperpolarized samples

David Lyndon Emsley, Geoffrey Bodenhausen, Sami Jannin

A method for the preparation of a hyperpolarized solution of molecules comprises the steps: 1) suspending or coating of a micro-particulate matrix, which is comprising or consisting of the molecules, with a glass-forming solution or suspension comprising a ...

2016

Hyperpolarization of Frozen Hydrocarbon Gases by Dynamic Nuclear Polarization at 1.2 K

David Lyndon Emsley, Geoffrey Bodenhausen, Aurélien Bornet, Sami Jannin, Jonas Milani, Basile Vuichoud, Estel Canet Martinez, David Benjamin Roger Antoine Gajan, David Baudouin

We report a simple and general method for the hyperpolarization of condensed gases by dynamic nuclear polarization (DNP). The gases are adsorbed in the pores of structured mesoporous silica matrices known as HYPSOs (HYper Polarizing SOlids) that have param ...

2016

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A method for the preparation of a sample comprising highly polarized nuclear spins is proposed, comprising at least the following steps: a) provision of molecules with 1,2-dione structural units and/or molecules with 2,5-diene-1,4-dione structural units in ...

2016

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We present novel means to hyperpolarize deuterium nuclei in (CD2)-C-13 groups at cryogenic temperatures. The method is based on cross-polarization from H-1 to C-13 and does not require any radio-frequency fields applied to the deuterium nuclei. After rapid ...

Amer Inst Physics2016

Observation of correlated spin-orbit order in a strongly anisotropic quantum wire system

Jan Hugo Dil, Stefan Peter Muff

Quantum wires with spin-orbit coupling provide a unique opportunity to simultaneously control the coupling strength and the screened Coulomb interactions where new exotic phases of matter can be explored. Here we report on the observation of an exotic spin ...

Nature Publishing Group2015

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Hyperpolarized nuclear spins are observed in optically pumped iron-doped InP from 70 K to 140 K. P-31 NMR was carried out at 9.28 T (159.8 MHz) during optical excitation with circularly polarized light, using a laser diode (lambda-830 nm) as a source. The ...

Academic Press Inc Elsevier Science2015