Engineering the Eigenstates of Coupled Spin-1/2 Atoms on a Surface
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Collective tunneling is a ubiquitous phenomenon in finite-size spin clusters that shows up in systems as diverse as molecular magnets or spin clusters adsorbed at surfaces. The basic problem we explore is to understand how small flipping terms can cooperat ...
This thesis presents a combined experimental and theoretical study of the classical and quantum magnetization dynamics in single magnetic adatoms and molecules, and on the classical and quantum coherent control thereof. First, a detailed description of the ...
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Strong quantum correlations in matter are responsible for some of the most extraordinary properties of materials, from magnetism to high-temperature superconductivity, but their integration in quantum devices requires a strong, coherent coupling with photo ...
2020
This thesis is devoted to the investigation of static and dynamic properties of
two different sets of quantum magnets with neutron scattering techniques and
the help of linear spin wave theory.
Both systems are copper-based with spin-1/2, which makes them ...
EPFL2021
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The thermal spin crossover (SCO) phenomenon refers to an entropy-driven spin transition in some materials based on d(6)-d(9) transition metal complexes. While its molecular origin is well known, intricate SCO behaviours are increasingly common, in which th ...
ROYAL SOC CHEMISTRY2020
The integrated network Mott Physics Beyond the Heisenberg Model (MPBH) united researchers across Switzerland in a collective effort to explore new aspects of Mott physics, in particular how spin-orbit interactions, in concert with strong electron correlati ...
The delafossite family of compounds with a triangular lattice of rare earth ions has been recently proposed as a candidate host for quantum spin liquid (QSL) states. To realize QSLs, the crystal electric field (CEF) ground state of the rare earth ions shou ...
Magnetic impurities generate a wealth of phenomena on surfaces. On metals, conducting electrons screen the magnetic moment giving rise to the Kondo effect. On superconductors, the Yu-Shiba-Rusinov (YSR) states emerge inside the superconducting gap due to t ...
We propose a practical implementation of a two-qubit entanglement engine which denotes a scheme to generate quantum correlations through purely dissipative processes. On a diamond platform, the electron spin transitions of two nitrogen-vacancy (NV) centers ...