Tunable few-optical cycle pulses and advanced ultrafast spectroscopic techniques
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In this paper, we study theoretically the generation of high repetition rate short pulses using fiber optical parametric amplification. We show that the pulse shape and duration depend on the signal location relatively to the pump frequency. We demonstrate ...
High-energy terahertz pulses are produced by optical rectification (OR) in organic crystals 4-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) and 4-N,N-dimethylamino-4'-N'-methyl-stilbazolium 2,4,6-trimethylbenzenesulfonate (DSTMS) by a Ti: sapphire ...
Multiferroics have attracted strong interest for potential applications where electric fields control magnetic order. The ultimate speed of control via magnetoelectric coupling, however, remains largely unexplored. Here, we report an experiment in which we ...
We report the development of an apparatus to allow time resolved photoelectron spectroscopy of charge motion on solids and structured surfaces with attosecond resolution in an ultra high vacuum environment. The system, connected to the Attosecond Beamline ...
In a recent study, the theory of pulse generation with fiber optical parametric amplification using sinusoidal (clock) intensity modulated pump was revisited [1]. This work showed that the pulses generated through such parametric interaction exhibit a shap ...
We demonstrate for the first time (to our knowledge) characterization of ultrashort IR pulses by self-referenced spectral interferometry. Both sub-55-fs pulses from 1.4 mu m to 2 mu m and broadband 2.5-cycle pulses at 1.65 mu m (13 fs FWHM) are characteriz ...
We demonstrate a cavity-less picosecond pulsed source near 2μm, tunable over more than 200nm based on third order cascaded Raman wavelength shifting. Up to 44% conversion is achieved for 100mW peak powers at 200MHz repetition rate. ...
A tunable, stable pulse generation technique based on two-pump fiber optic parametric amplification is theoretically analyzed and experimentally demonstrated to generate uniform near-Gaussian pulses over 32 nm. It is shown that pulse shape can also be tune ...
We present a broadband two-dimensional transient absorption setup for the UV around 300 nm with a time resolution of 150 fs. A narrowband, frequency tunable pump pulse and a broadband probe pulse are generated from the output of a noncollinear optical para ...
We describe a complete technological system at Imperial College London for Attosecond Science studies. The system comprises a few-cycle, carrier envelope phase stabilized laser source which delivers sub 4 fs pulses to a vibration-isolated attosecond vacuum ...