Publication

Second Harmonic Generation Dynamics in Plasmonic Nanoparticles

Olivier Martin, Jérémy Butet, Gabriel David Bernasconi
2018
Conference paper

Abstract

Due to its symmetry properties, second-harmonic generation in plasmonic nanostructures enables the observation of even-parity modes that couple weakly to the far field. Consequentially, those modes radiate less and thus have a longer lifetime. Using a full-wave numerical method, we study the linear and second harmonic dynamical responses of a silver nanorod under plane-wave femtosecond pulse illumination. Depending on the spectral position and duration of the pulse, the decaying field of the different modes can be separated, and the free oscillations of each mode are well fitted by a damped harmonic oscillator model, both in the linear and nonlinear regimes. Additionally, interference effects between different modes excited at the second harmonic are observed.

Official source

https://infoscience.epfl.ch/record/262573?ln=en

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Related concepts (32)

Harmonic oscillator

In classical mechanics, a harmonic oscillator is a system that, when displaced from its equilibrium position, experiences a restoring force F proportional to the displacement x: where k is a positive constant. If F is the only force acting on the system, the system is called a simple harmonic oscillator, and it undergoes simple harmonic motion: sinusoidal oscillations about the equilibrium point, with a constant amplitude and a constant frequency (which does not depend on the amplitude).

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High harmonic generation (HHG) is a non-linear process during which a target (gas, plasma, solid or liquid sample) is illuminated by an intense laser pulse. Under such conditions, the sample will emit the high harmonics of the generation beam (above the fifth harmonic). Due to the coherent nature of the process, high harmonics generation is a prerequisite of attosecond physics. Perturbative harmonic generation is a process whereby laser light of frequency ω and photon energy ħω can be used to generate new frequencies of light.

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