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Competition between intermediate plaquette phases in SrCu2(BO3)(2) under pressure

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Inelastic Neutron Scattering for Néel Phase Excitation Spectrum of SrCu2(BO3)2

Martin Tang Bruland

Spin excitations in the antiferromagnetic Néel phase of the Shastry-Sutherland crystal SrCu2(BO3)2 have been investigated using inelastic neutron scattering. No clear excitations could be identified, possibly due to challenging experimental conditions ulti ...

2023

Investigating field-induced magnetic order in Han purple by neutron scattering up to 25.9 T

Frédéric Mila, Bruce Normand, Philippe Heller, Nicolas Laflorencie

BaCuSi2O6 is a quasi-two-dimensional (2D) quantum antiferromagnet containing three different types of stacked, square-lattice bilayer hosting spin-1/2 dimers. Although this compound has been studied extensively over the last two decades, the critical appli ...

AMER PHYSICAL SOC2022

Small-angle neutron scattering study of mesoscale magnetic disordering and skyrmion phase suppression in the frustrated chiral magnet Co6.75Zn6.75Mn6.51

Henrik Moodysson Rønnow, Jonathan White

Co-Zn-Mn chiral cubic magnets display versatile magnetic skyrmion phases, including equilibrium phases stable far above and far below room temperature, and the facile creation of robust far-from-equilibrium skyrmion states. In this system, compositional di ...

INT UNION CRYSTALLOGRAPHY2022

Static and dynamic properties of non-collinear quantum antiferromagnets explored by neutron scattering

Luc Testa

This thesis is devoted to the investigation of static and dynamic properties of two different sets of quantum magnets with neutron scattering techniques and the help of linear spin wave theory. Both systems are copper-based with spin-1/2, which makes them ...

EPFL2021

Ferrimagnetic 120 degrees magnetic structure in Cu2OSO4

Henrik Moodysson Rønnow, Arnaud Magrez, Ivica Zivkovic, Nicola Casati, Helmuth Berger, Lin Yang, Gregory Scott Tucker, Virgile Yves Favre, Romain Sibille

We report magnetic properties of a 3d(9) (Cu2+) magnetic insulator Cu2OSO4 measured on both powder and single crystal. The magnetic atoms of this compound form layers whose geometry can be described either as a system of chains coupled through dimers or as ...

AMER PHYSICAL SOC2020

Multiphase magnetism in Yb2Ti2O7

Gregory Scott Tucker

We use neutron scattering to show that ferromagnetism and antiferromagnetism coexist in the low T state of the pyrochlore quantum magnet Yb2Ti2O7. While magnetic Bragg peaks evidence long-range static ferromagnetic order, inelastic scattering shows that sh ...

NATL ACAD SCIENCES2020

Nuclear Quantum Effects: Fast and Accurate

Venkat Kapil

Atomistic simulations are a bottom up approach that predict properties of materials by modelling the quantum mechanical behaviour of all electrons and nuclei present in a system. These simulations, however, routinely assume nuclei to be classical particles ...

EPFL2020

We report that Cu9O2(SeO3)(4)Cl-6 is a new multiferroic compound. Comprehensive studies of this compound have been carried out on single crystals as well as polycrystalline samples. Magnetic susceptibility chi and specific heat C with H parallel to c axis ...

AMER PHYSICAL SOC2019

Weak Crystallization of Fluctuating Skyrmion Textures in MnSi

Dirk Grundler

We report an experimental study of the emergence of nontrivial topological winding and long-range order across the paramagnetic-to-skyrmion lattice transition in the transition metal helimagnet MnSi. Combining measurements of the susceptibility with small- ...

2019

Collective magnetic excitations are a fascinating aspect of condensed matter physics, where neutron scattering can provide valuable insight into the magnetic properties of physical realisations of model systems. This thesis focuses on the excitation spectr ...

EPFL2017