A mm(3) Fiber-Coupled Scintillator for In-Core Thermal Neutron Detection in CROCUS

This article presents the development, full-characterization, and in-core testing of a miniature neutron detector for the investigation of highly localized in-core neutronics effects in the zero-power reactor CROCUS, operated at the Ecole Polytechnique federale de Lausanne (EPFL), Switzerland. A ZnS:(LiF)-Li-6 screen, mixing inorganic scintillator and neutron converter, with a surface of 1 mm(2) and a thickness of 0.2 mm, was coupled with a silicon photomultiplier (SiPM) via a 10-m optical fiber. Analog readout electronics were adopted in this prototype version to process the SiPM output signal. A first campaign was carried out to assess the detection system capabilities in terms of neutron detection and counting in mixed neutron-gamma radiation fields. The miniature detector was thoroughly characterized with a Pu-Be source installed in the CARROUSEL facility and was subsequently tested inside a control rod guide tube of the CROCUS reactor in different reactor conditions, i.e., at shutdown, startup, and critical. The detector shows a linear response with a reactor power increase up to 6.5 W (i.e., around 108 cm(-2) . s(-1) total neutron flux) and excellent neutron counting capabilities, when compared to other localized detection systems available in CROCUS, such as the miniature fission chambers and single-crystal vapor deposited (sCVD) diamond detectors. In addition, the exposure of the miniature detector to a Co-60 source with an activity of similar to 250 GBq, combined with the computation of the gamma flux in CROCUS with the Serpent 2 Monte Carlo code, confirmed the gamma insensitivity of the system in a mixed neutron-gamma field.

Design and Simulation of Gamma Spectrometry Experiments in the CROCUS Reactor

Mathieu Hursin, Vincent Pierre Lamirand, Oskari Ville Pakari, Andreas Pautz, Fanny Vitullo

Gamma rays in nuclear reactors, arising either from fission or decay processes, significantly contribute to the heating and dose of the reactor components. Zero power research reactors offer the possibility to measure gamma rays in a purely neutronic environment, allowing for validation experiments of computed spectra, dose estimates, reactor noise and prompt to delayed gamma ratios. This data then contributes to models, code validation and photo atomic nuclear data evaluation. In order to contribute to aforementioned experimental data, gamma detection capabilities are being added to the CROCUS reactor facility. The CROCUS reactor is a two-zone, uranium-fueled light water moderated facility operated by the Laboratory for Reactor Physics and Systems Behaviour (LRS) at the Swiss Federal Institute of Technology Lausanne (EPFL). With a maximum power of 100 W, it is a zero power reactor used for teaching and research, most recently for intrinsic and induced neutron noise studies. For future gamma detection applications in the CROCUS reactor, an array of four detectors - two large 5 '' x10 '' Bismuth Germanate (BGO) and two smaller Cerium Bromide (CeBr3) scintillators - was acquired. The BGO detectors are to be arbitrarily positioned in the core reflector and out of the vessel for measurements at arbitrary distances. The CeBr3 detectors on the other hand are small enough to be set in the guide tubes of the control rods for in-core measurements. We present a study of the neutron and gamma flux in the core and reflector using the MCNP 6.2 and Serpent 2 Monte Carlo codes for coupled neutron and photon transport criticality calculations. More specifically, we investigate and compare predicted spectra as well as reactivity worth of different envisioned experimental setups. We further predict pulse height spectra as well as doses to the crystals with and without cadmium shielding to estimate allowable reactor powers with respect to detector radiation hardness. The results serve as basis for calibration and aid in the design and regulatory approval of the experiments.

E D P SCIENCES2020

Development of the control assembly pattern and dynamic analysis of the generation IV large gas-cooled fast reactor (GFR)

Gaëtan Girardin

During the past ten years, different independent factors, such as the rapidly increasing worldwide demand in energy, societal concerns about greenhouse gas emissions, and the high and volatile prices for fossil fuels, have contributed to the renewed interest in nuclear technology. It is in this context that the Generation IV international forum (GIF) launched the initiative, in 2000, to collaborate on the research and development (R&D) efforts needed for the next generation, i.e. Generation IV, of nuclear reactors. These advanced systems will be ideally deployed beyond the year 2030, following the Generation III or III+ nuclear power plants, which are mainly based on light water technology and are currently entering deployment. A particular goal set for Generation IV systems is closure of the nuclear fuel cycle. Thus, apart from improvements in safety, they are expected to offer a better utilization of natural resources, as also a minimization of long-lived radioactive wastes. Among the systems selected by the GIF, the Gas-cooled Fast Reactor (GFR) is a highly innovative system with advanced fuel geometry and materials (fuel pellets of mixed uranium-plutonium carbide within a plate-type, honeycomb structure made of SiC). It is in the context of the large, 2400 MWth reference GFR design that the present doctoral research has been conducted, the principal aim having been to develop and qualify the control assembly (CA) pattern and corresponding CA implementation scheme for this system. The work has been carried out in three successive and complementary phases: (1) validation of the neutronics tools, (2) the CA pattern development and related static analysis, and (3) dynamic core behavior studies for hypothetical CA driven transients. The deterministic code system ERANOS and its associated nuclear data libraries for fast reactors were developed and validated for the previous generation of sodium-cooled reactors. The validation of ERANOS for GFR applications was, therefore, the first task to be realized in the present research. This has entailed a systematic reanalysis of the GFR-relevant, integral data generated at PSI during the GCFR-PROTEUS experimental program of the 1970's. Thus, during the first phase of the thesis, the reference PROTEUS test lattice from these experiments has been analyzed with ERANOS-2.0 and its associated, adjusted nuclear data library ERALIB1, in order to derive a reference computational scheme to be used later for the GFR analysis. Additionally, benchmark calculations were performed with the Monte Carlo code MCNPX, allowing one to both check the deterministic results and to analyze the sensitivity to different modern data libraries. It has been found that, for the main reaction rate ratios, the new analysis of the GCFR-PROTEUS reference lattice generally yields good agreement – within 1σ measurement uncertainty – with experimental values and with the Monte Carlo simulations. As shown by the analysis, the predictions were in somewhat better agreement in the case of the adjusted ERALIB1 library. The applicability of ERANOS-2.0/ERALIB1 as the reference neutronics tool for the GFR analysis could thus be demonstrated. Furthermore, neutronics aspects related to the novel features of the GFR, for which new experimental investigations are needed, were highlighted. In the second phase of the research, the CA pattern was developed for the GFR, based on iterative neutronics and thermal-hydraulics calculations, 2D and 3D neutronics models for the reactor core having first been set up using the reference ERANOS-2.0/ERALIB1 computational scheme. For the thermal-hydraulics analysis, the CEA code COPERNIC was used. This design work was followed by the study of an appropriate CA implementation scheme (number of CAs and corresponding positions within the core). Detailed neutronics studies revealed the existence of large CA interaction effects, so-called shadowing/anti-shadowing effects leading to an amplification/reduction of the CA worth. The interactions between the absorber pins within a CA, and between the CAs themselves, were investigated in detail, with the goal to optimize the CA efficiency, in terms of the absorber fraction and minimization of the associated heterogeneity effects. The proposed CA pattern consists of 54 absorber pins placed in a triangular lattice. Each absorber pin is a stainless-steel tube filled with highly enriched 10B boron carbide pellets. As a result of the detailed investigations, the absorber pin diameter could be chosen such as to minimize the pin-to-pin influence within the assembly. In particular, a central part of the CA was designed without any absorber pins (zone filled with stagnant helium). A final reduction of the heterogeneity effect (difference between homogeneous and heterogeneous treatments) to 13% was achieved through this feature. Of special importance, the neutronics investigations performed for the reference GFR core ("2004-Core"), especially those related to the CA interactions, have directly contributed to a new core design ("2007-Core"), with the height-to-diameter ratio having been increased to 0.6, compared to 0.3 for the reference core. During the third phase, detailed coupled, 3D neutron-kinetics (NK) and 1D thermal-hydraulics (TH) models were developed for the GFR core, the aim being to arrive at an in-depth understanding of the 3D core behavior during CA driven transients, especially from the viewpoint of spatial effects. The coupled models were developed using the PARCS code for the 3D NK and the TRACE code for the 1D TH modeling. Particular attention was paid to have each individual fuel sub-assembly and CA represented, in order to allow the analysis of local deformations of the 3D distributions of power and safety related parameters, such as the coolant, cladding and fuel temperatures. The validation of the coupled full-core models was performed against reference ERANOS-VARIANT calculations. In particular, the CA worth and reactivity feedbacks were benchmarked, the discrepancies being shown to be relatively low (

EPFL2009

Modeling the response of a diamond detector in the zero power reactor CROCUS

Pavel Frajtag, Mathieu Hursin, Vincent Pierre Lamirand, DongHyuk Lee, Andreas Pautz

The present manuscript documents the development of a practical calculation scheme to model the response of a diamond detector in the mixed (neutron and gamma) radiation field of the CROCUS experimental reactor at EPFL. The model is shown to perform reasonably well in terms of energy spectra shapes for the limited amounts of irradiations considered; the relative magnitude of the neutron and gamma contributions to the detector output is, however, not properly captured. The gamma contribution is underestimated by a factor of four if the neutron contribution is correctly captured. A sensitivity study to three parameters (the azimuthal position of the detector, the magnitude of the neutron and gamma sources, and the threshold voltage used in the detector) is also carried out to analyze the effect of modeling assumptions and experimental choices on the results. Then, a detailed analysis of the computational results is carried out to provide quantitative information about the response of a diamond detector in a mixed radiation field. It is shown that the low-energy interactions are mainly produced by gamma interactions; that the high energy interactions are generated by proton recoil interactions; and that 60% of the recorded neutron interactions are produced by thermal neutron captures in Li-6, while the rest come from scattering interactions with fast neutrons. Finally, it is demonstrated that considering some of the effects of the electronics on the pulses (RC time constant) is required to reproduce the trends observed in the experimental results, especially the increased detection rate within the diamond crystal.