Direct observation of non-fully-symmetric coherent optical phonons by femtosecond x-ray diffraction

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Electronic Population Transfer via Impulsive Stimulated X-Ray Raman Scattering with Attosecond Soft-X-Ray Pulses

Christoph Bostedt, Xiang Li, Andre Al Haddad, Solène Oberli, Siqi Li

Free-electron lasers provide a source of x-ray pulses short enough and intense enough to drive nonlinearities in molecular systems. Impulsive interactions driven by these x-ray pulses provide a way to create and probe valence electron motions with high tem ...

AMER PHYSICAL SOC2020

Imaging plasma formation in isolated nanoparticles with ultrafast resonant scattering

Christoph Bostedt, Daniela Rupp, Alessandro Colombo

We have recorded the diffraction patterns from individual xenon clusters irradiated with intense extreme ultraviolet pulses to investigate the influence of light-induced electronic changes on the scattering response. The clusters were irradiated with short ...

2020

Peculiarities of second harmonic generation with chirped femtosecond pulses at high conversion efficiency

Pierre-Marc Jean Marie Dansette

Frequency doubling of an infrared laser radiation in non-linear optical crystals is a widely used technique to obtain light in the visible range. The second harmonic generation process is influenced by several well-known parameters. In this article we stud ...

ELSEVIER2020

Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

Christoph Bostedt, Zhaoheng Guo, Jonas Knurr, Andre Al Haddad, Siqi Li

The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray t ...

ROYAL SOC CHEMISTRY2020

Spectral Properties of the Signal in Phase-Sensitive Optical Time-Domain Reflectometry with Direct Detection

Luc Thévenaz, Marcelo Alfonso Soto Hernandez, Li Zhang, Xin Lu

The spectral properties of the Rayleigh backscattered traces measured by a phase-sensitive optical time-domain reflectometer (øOTDR) with direct detection are theoretically and experimentally analyzed. The spectrum of the measured øOTDR signal is found to ...

IEEE Institute of Electrical and Electronics Engineers2020

Tracking attosecond electronic coherences using phase-manipulated extreme ultraviolet pulses

Marcel Drabbels, Primoz Rebernik Ribic

The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear spectroscopy schemes ...

Nature Research2020

Modes interplay controls the second harmonic generation dynamics of plasmonic nanostructures

Olivier Martin, Andrei Kiselev, Gabriel David Bernasconi

A large amount of experimental and theoretical works deals with the second harmonic generation from different plasmonic geometries. Since they often consider relatively long optical pulses, many of these studies are focused on the investigation of a quasi- ...

SPIE2020

Ultrafast relaxation of photoexcited superfluid He nanodroplets

Marcel Drabbels, Alberto Hernando de Castro

The relaxation of photoexcited nanosystems is a fundamental process of light–matter interaction. Depending on the couplings of the internal degrees of freedom, relaxation can be ultrafast, converting electronic energy in a few fs, or slow, if the energy is ...

Nature Research2020

Generating optical pulses via a soliton state of an optical microresonator coupled with a chip based semiconductor laser

Tobias Kippenberg, Hairun Guo, Arslan Sajid Raja

A light pulse source (100), being adapted for generating repetitive optical pulses (1), comprises a continuous wave cw laser device (10) being arranged for providing cw laser light (2), an optical waveguide (20) being optically coupled with the cw laser de ...

2020

Ultra-broadband time-resolved THz spectroscopy of perovskites and nanomaterials

Andrés Burgos Caminal

The fundamental study of charge carrier dynamics has been shown to be of great interest for optoelectronics, paving the way forward for future developments. Often, some of the key processes that determine the photophysics of a material occur on very short ...

EPFL2020

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