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We explain how and under which conditions it is possible to obtain an efficient inversion of an entire sideband family of several hundred kHz using low-power, sideband-selective adiabatic pulses, and we illustrate with some experimental results how this fr ...
Multiple refocusing cycles can be used to extract transverse relaxation rates, R2, while homonuclear scalar couplings do not interfere. In this work, I have demonstrated the usefulness of a hybrid sequence, which is a compromise between single and multiple ...
A train of short rotor-synchronized pulses in the manner of Delays Alternating with Nutations for Tailored Excitation (DANTE) applied to nitrogen-14 nuclei (I = 1) in samples spinning at the magic angle at high frequencies (typically nu(rot) = 62.5 kHz so ...
Vibrational sum-frequency generation (SFG) employing femtosecond infrared (IR) laser pulses is used to study the dynamics of the C-O stretch vibration on Ru(0 0 1). Time-resolved measurements of the free induction decay (FID) of the IR-polarization for 0.3 ...
The high intrinsic spin and long spin relaxation time of manganese-12-acetate (Mn-12) makes it an archetypical single molecular magnet. While these characteristics have been measured on bulk samples, questions remain whether the magnetic properties replica ...
Nuclear Magnetic Resonance (NMR) spectroscopy offers many ways to investigate dynamic properties of molecules. A wide variety of experimental techniques can probe molecular dynamics on time scales that range from 10-12 to 103 seconds. Many lines of evidenc ...
It is shown how transverse magnetization can be excited with a single low-power radiofrequency pulse consisting of a superposition of 2 frequency-modulated components. The phase dispersion obtained with this self-refocusing pulse is very small over bandwid ...
Since many biological processes occur on the μs to ms time scale, internal dynamics on that time scale may well be related to biological functionality. The characterization of internal dynamics is thus an important issue to improve our understanding of the ...
This paper presents the implementation of the 1.2 mm2 HSDPA turbo decoder ASIC in 0.13 mum CMOS achieves a measured maximum frequency of 246 MHz, which translates to a maximum throughput of 20.2 Mb/s at 5.5 iterations. The peak throughput of 10.8 Mb/s requ ...
In NMR of spins with I = 1/2 in an isotropic phase, it is demonstrated by simulation and expt. that virtually unlimited bandwidths can be decoupled effectively by using chirp pulses with linear frequency modulation for adiabatic inversion combined with pha ...
