"Bubble" dynamics following Rydberg state excitation in rare gas matrixes
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Higher Rydberg states of NO trapped in rare gas matrixes were studied by inducing Rydberg-Rydberg transitions from the lowest A2S+ (3ss) Rydberg state and detecting its fluorescence depletion. This technique unravels Rydberg states, which cannot be accesse ...
Excitation of the A(3ss) Rydberg state of NO trapped in an H2 crystal leads to the electronic bubble formation around the NO impurity, resulting in an increase of 0.9 .ANG. of the ground state cage radius. Its dynamics was followed in real-time by femtosec ...
