Efficient Stimulated Raman Pumping for Quantum-State Resolved Surface Reactivity Measurements
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Using a density-functional framework, we investigate the vibrational spectra of vitreous SiO2 to determine to what extent these spectra provide information about the medium-range structure of the oxide network. We carry out a comparative study involving th ...
We present a method for determining molecular orientation from second-order nonlinear light scattering experiments. Our modeling shows that there is an optimal angular region, for which the scattering pattern is most sensitive to molecular orientation. We ...
We report the first 320-Gb/s all-optical wavelength multicast experimental demonstration in two-pump parametric amplifier, assisted by pump-pump self seeding. A single 320-Gb/s channel was successfully multicast to eight wavelengths with minimal conversion ...
Institute of Electrical and Electronics Engineers2009
Infrared absorption spectroscopy enabling direct access to vibrational fingerprints of the molecular structure is a powerful method for functional studies of bio-molecules. Although the intrinsic absorption cross-sections of IR active modes of proteins are ...
Raman spectra are presented for the rare-earth nitrides SmN, GdN, DyN, ErN, and LuN measured with 633 and 514 nm excitation wavelengths and at temperatures above and below the Curie temperature. Frozen-phonon calculations are presented for the phonons at G ...
In this paper we propose the use of multi-longitudinal mode lasers, such as Fabry-Pérot (FP) lasers, for simultaneous distributed strain and temperature sensing based on hybrid Brillouin and Raman scattering. Fabry-Pérot lasers allow for high-power Raman i ...
Using the Submillimeter Array we have detected the J = 3-2 and 2-1 rotational transitions from within the first vibrationally excited state of CO toward the extreme carbon star IRC+10216 (CW Leo). The emission remains spatially unresolved with an angular r ...
We present here the analysis of experimental Stark effect measurements made using photofragment quantum beat spectroscopy on the 14,0->, 15,0->, 18,0+> and 14,0-> 12 > vibrational states of H2O [Callegari, A.; et al. Science 2002, 297, 993.]. To link the m ...
Many processes in chemistry and physics rely on the structure, growth or change of material buried in solids. The impenetrable surrounding medium often prohibits the study of such material in situ. Nonlinear light scattering can be used to observe the inte ...
We report, for the first time, simultaneous wavelength conversion for WDM multicasting of an optical time division multiplexed single data channel at 320 Gb/s using a 2-pump fiber optic parametric amplifier. ...