Mass-selected deposition of Ag 7 on Pd(100). Evidence for implantation and strong fragmentation
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I present a molecular beam study of methane dissociation on differ-ent surface sites of several platinum single crystal surfaces (Pt(111), Pt(211), Pt(210), Pt(110)-(2x1)). The experiments were performed in a molecular beam/surface-science apparatus that c ...
In my thesis, I present an investigation of the dissociation reactions of gas phase molecules on single crystal metal surfaces studied by a molecular beam in combination with Reflection Absorption Infrared Spectroscopy (RAIRS). Two gas/surface systems were ...
Partial autoionization rates of doubly excited one-dimensional helium in the collinear Zee and eZe configuration are obtained by means of the complex rotation method. The approach presented here relies on a projection of back-rotated resonance wave functio ...
The spatial volume occupied by an atom depends on its electronic density. Although this density can only be evaluated exactly for hydrogen-like atoms, there are many excellent algorithms and packages to calculate it numerically for other materials. Three-d ...
Solid-liquid interfaces are ubiquitous. Despite the unquestioned relevance, many scientific research fields rely on simplified or macroscopic descriptions, discarding the molecular nature of the constituents. However, it is the specific molecular interacti ...
Traditional neutron tomography allows to reconstruct the attenuation cross section, a measure for the material distribution, at high spatial resolution and non-destructively. However, it does not state anything about the ordering structure of the atoms ins ...
The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms pro ...
The electron microscopy community makes a wide use of Energy Dispersive X-ray Spectrometry (EDS) for elemental mapping in STEM. This technique was however long reckoned slow, dozens of minutes if not an hour, to collect enough information for one map. Rece ...
The microscopic description of the interface of colloidal particles in solution is essential to understand and predict the stability of these systems, as well as their chemical and electrochemical reactivity. However, this description often relies on the u ...
Biological pathways have been extensively analyzed and modeled in respect to overall conversions of substrates to products, although information on atom transitions or atom flow in metabolic networks is not available in databases. The reaction atom mapping ...
