Procédé kraft

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Techno-economic analysis and life cycle assessment of a biorefinery utilizing reductive catalytic fractionation

Jeremy Luterbacher

Reductive catalytic fractionation (RCF) is a promising approach to fractionate lignocellulose and convert lignin to a narrow product slate. To guide research towards commercialization, cost and sustainability must be considered. Here we report a techno-eco ...

2021

Potential of hydrothermal black liquor gasification integrated in pulp production plant

François Maréchal, Julia Granacher, Maziar Kermani, Ayse Dilan Celebi

Greenhouse gas emission mitigation is one of the main motivations for increasing the use of biomass in providing environmentally friendly value-added products. The pulp and paper industry is a promising sector for the integration of biorefinery pathways. A ...

Silesian University of Technology2019

Fractionation of lignocellulosic biomass to produce uncondensed aldehyde-stabilized lignin

Jeremy Luterbacher, Masoud Talebi Amiri, Ydna Marie Questell-Santiago, Graham Reid Dick

Lignin is one of the most promising sources of renewable aromatic hydrocarbons. Current methods for its extraction from lignocellulosic biomass—which include the kraft, sulfite, and organosolv processes—result in the rapid formation of carbon–carbon bonds, ...

2019

Preventing Lignin Condensation to Facilitate Aromatic Monomer Production

Jeremy Luterbacher, Wu Lan

Lignin is the most abundant aromatic polymer in nature and as such is an attractive source of aromatic molecules. Efficient lignin utilization will also likely play a key role in the economic success and sustainability of biomass valorization schemes. Howe ...

2019

Production and characterization of stabilized lignin

Masoud Talebi Amiri

Lignocellulosic biomass is a sustainable source of renewable carbon, and it is the most abundant form of terrestrial biomass. The three main constituents of lignocellulosic biomass are cellulose, hemicellulose, and lignin. The monomers from these biopolyme ...

EPFL2019

Topology of Pretreated Wood Fibers Using Dynamic Nuclear Polarization

David Lyndon Emsley, Jeremy Luterbacher, Arthur César Pinon, Pierrick Berruyer, Jasmine Viger-Gravel, Wu Lan, Michel Bardet

In the continuously developing field of lignocellulosic biomass, high-yield lignin depolymerization processes are sought to optimize its productivity and profitability. Recently, formaldehyde stabilization during lignin extraction and biomass pretreatment ...

2019

A Holistic Methodology for Optimizing Industrial Resource Efficiency

François Maréchal, Adriano Viana Ensinas, Ivan Daniel Kantor, Julia Granacher, Maziar Kermani, Anna Sophia Wallerand

Efficient consumption of energy and material resources, including water, is the primary focus for process industries to reduce their environmental impact. The Conference of Parties in Paris (COP21) highlighted the prominent role of industrial energy effici ...

2019

Protection Group Effects During α,γ-Diol Lignin Stabilization Promote High-Selectivity Monomer Production

Jeremy Luterbacher, Wu Lan, Masoud Talebi Amiri, Christopher Marc Hunston

Protection groups were introduced during biomass pretreatment to stabilize lignin's α,γ-diol group during its extraction and prevent its condensation. Acetaldehyde and propionaldehyde stabilized the α,γ-diol without any aromatic ring alkylation, which sign ...

Wiley-VCH Verlag GmbH2018

Methodologies for simultaneous optimization of heat, mass, and power in industrial processes

Maziar Kermani

EPFL2018

Formaldehyde stabilization facilitates lignin monomer production during biomass depolymerization

Jeremy Luterbacher, Yiming Li, Florent Emmanuel Héroguel, Masoud Talebi Amiri, Ydna Marie Questell-Santiago, Li Shuai

Practical, high-yield lignin depolymerization methods could greatly increase biorefinery productivity and profitability. However, development of these methods is limited by the presence of interunit carbon-carbon bonds within native lignin, and further by ...

American Association for the Advancement of Science2016

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