Concept

Diffusion inélastique de rayonnement

Publications associées (87)

Spin-gap evolution upon Ca doping in the spin-ladder series Sr(14−x)CaxCu24O41 studied by inelastic neutron scattering

Henrik Moodysson Rønnow, Nikolay Tsyrulin, Kazimierz Conder

The spin-gap evolution upon Ca doping in Sr14-xCaxCu24O41 was systematically investigated using inelastic neutron scattering. We discover that the singlet-triplet spin-gap excitation survives in this series with x up to 13, indicating the singlet dimer gro ...

American Physical Society2013

Glassy low-energy spin fluctuations and anisotropy gap in La1.88Sr0.12CuO4

Henrik Moodysson Rønnow, Joël Mesot, Johan Juul Chang

We present high-resolution triple-axis neutron scattering studies of the high-temperature superconductor La1.88Sr0.12CuO4 (Tc=27 K). The temperature dependence of the low-energy incommensurate magnetic fluctuations reveals distinctly glassy features. The g ...

American Physical Society2013

Origin of the large anharmonicity in the phonon modes of LiBH4

The dynamics and bonding of the complex hydride LiBH4 have been investigated by vibrational spectroscopy and density functional theory (DFT). The combination of infrared, Raman, and inelastic neutron-scattering (INS) spectroscopies on hydrided and deuterat ...

2013

Development of the magnetic excitations of charge-stripe ordered La2-xSrxNiO4 on doping towards checkerboard charge order

Paul Gregory Freeman

The magnetic excitation spectrums of charge stripe ordered La2-x Sr (x) NiO4 x = 0.45 and x = 0.4 were studied by inelastic neutron scattering. We found the magnetic excitation spectrum of x = 0.45 from the ordered Ni2+ S = 1 spins to match that of checker ...

Korean Physical Soc2013

Glassy low-energy spin fluctuations and anisotropy gap in La_{1.88}Sr_{0.12}CuO_{4}

Joël Mesot, Johan Juul Chang, Christopher Werner Matthias Robeller

We present high-resolution triple-axis neutron scattering studies of the high-temperature superconductor La1.88Sr0.12CuO4 (T-c = 27 K). The temperature dependence of the low-energy incommensurate magnetic fluctuations reveals distinctly glassy features. Th ...

Amer Physical Soc2013

The Fuzzy Quantum Proton in the Hydrogen Chloride Hydrates

Michele Ceriotti, Michele Parrinello

The motion of the excess proton is understood as a process involving interconversion between two limiting states, namely, the Eigen and Zundel cations. Nuclear quantum effects (NQE) and the organization of the surrounding solvent play a significant role in ...

2012

Hydrogen adsorption in the metal-organic frameworks Fe2(dobdc) and Fe2(O2)(dobdc)

Wendy Lee Queen

The hydrogen storage properties of Fe2(dobdc) (dobdc4- = 2,5-dioxido-1,4-benzenedicarboxylate) and an oxidized analog, Fe2(O2)(dobdc), have been examd. using several complementary techniques, including low-pressure gas adsorption, neutron powder diffractio ...

2012

Simultaneous measurement of lithium and fluorine momentum in

Michele Ceriotti

We present momentum widths and mean kinetic energies of lithium and fluorine in 7LiF, as determined simultaneously from deep inelastic neutron scattering (DINS) measurements. Experimental data across a temperature range from 4 to 300K are presented, and th ...

2012

Inelastic Scatterings and Applications to Distributed Sensing

Luc Thévenaz

Inelastic scatterings turn out to occupy an essential place in sensing applications, since they simply require a plain optical fibre as sensing element, with no special preparation. They give rise to energy and momentum transfers with the fibre material an ...

EPFL Press, distributed by CRC Press2011

Experimental evidence of librational vibrations determining the stability of calcium borohydride

Pascal Martelli

The high energy of hydrogen vibrations in solids is the origin of their strong impact on thermodynamic properties. The peculiar structure of complex hydrides amplifies this impact. We shed light on the vibrational properties of three allotropes of Ca(BH4)2 ...

2011

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