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The splitting of water into hydrogen and oxygen molecules using sunlight is an attractive method for solar energy storage. Until now, photoelectrochemical hydrogen evolution is mostly studied in acidic solutions, in which the hydrogen evolution is more fac ...
A fundamental requirement for a renewable energy generation technology is that it should produce more energy during its lifetime than is required to manufacture it. In this study we evaluate the primary energy requirements of a prospective renewable energy ...
A validated multi-physics numerical model that accounts for charge and species conservation, fluid flow, and electrochemical processes has been used to analyze the performance of solar-driven photoelectrochemical water-splitting systems. The modeling has p ...
The actualization of a hydrogen economy requires cost-effective and environmentally benign solutions to hydrogen production. Chemical energy in the form of hydrogen is more interesting than electricity to satisfy our ever-increasing energy demand because i ...
The instantaneous efficiency of an operating photoelectrochemical solar-fuel-generator system is a complicated function of the tradeoffs between the light intensity and temperature-dependence of the photovoltage and photocurrent, as well as the losses asso ...
Devices that directly capture and store solar energy have the potential to significantly increase the share of energy from intermittent renewable sources. Photo-electrochemical solar-hydrogen generators could become an important contributor, as these devic ...
In order to be economically competitive with simple "brute force" (i.e., PV + electrolyzer) strategies or the production of promising solar fuels, like H-2, from fossil fuels, a practical photoelectrochemical device must optimize cost, longevity, and perfo ...
