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Concept

Résonance paramagnétique électronique

Science de la nature
Chimie
Chimie physique
Spectroscopie

Publications associées (1 000)

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Publications associées (1 000)

A Mesoionic Diselenolene Anion and the Corresponding Radical Dianion

Rosario Scopelliti, Kay Severin, Farzaneh Fadaei Tirani, Andrzej Sienkiewicz, Abdusalom Suleymanov, Zhaowen Dong, Cesare Berton

Dichalcogenolenes are archetypal redox non-innocent ligands with numerous applications. Herein, we describe a diselenolene ligand with fundamentally different electronic properties. By selenation of a C2-protected imidazolium salt, we have prepared a mesoi ...

2022

A Low Power 35 GHz HEMT Oscillator for Electron Spin Resonance Spectroscopy

Giovanni Boero, Nergiz Sahin Solmaz, Alessandro Valentino Matheoud

This paper presents a low power microwave oscillator designed as sensor for electron spin resonance (ESR) spectroscopy. Low power consumption is necessary for low temperature operation. Additionally, lower power consumption allows for a lower microwave mag ...

IEEE2021

Core-Valence Attosecond Transient Absorption Spectroscopy of Polyatomic Molecules

Jiri Vanicek, Nikolay Golubev

Tracing ultrafast processes induced by interaction of light with matter is often very challenging. In molecular systems, the initially created electronic coherence becomes damped by the slow nuclear rearrangement on a femtosecond timescale which makes real ...

2021

FEM simulation: Thermal properties of thin film quartz and silicon resonators

This semester project aimed at simulating two approaches for low temperature dependence of resonance frequency of resonators. The first one consists in using AT-cut quartz as the resonator’s material. The AT-cut quartz wafers are made using a 35° angle wit ...

2021

Tuning interactions in reconfigurable kagome artificial spin ices for magnonics

Dirk Grundler, Vinayak Shantaram Bhat

We report broadband spin-wave spectroscopy on kagome artificial spin ices (KASIs) made of large arrays of disconnected Ni81Fe19 400-nm-long nanobars. We observed spin wave spectra that varied characteristically upon the separation between neighboring nanob ...

2021

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O-17 NMR is an invaluable tool to study the structure and dynamics of oxide materials but remains challenging to apply in many systems. Even with isotopic enrichment, studies of samples with low masses and/or concentrations of the active species, such as t ...

AMER CHEMICAL SOC2021

Confined dipole and exchange spin waves in a bulk chiral magnet with Dzyaloshinskii-Moriya interaction

Dirk Grundler, Ping Che, Andrea Mucchietto, Helmuth Berger, Jianing Li

The Dzyaloshinskii-Moriya interaction (DMI) has an impact on excited spin waves in the chiral magnet Cu2OSeO3 by means of introducing asymmetry in their dispersion relations. The confined eigenmodes of a chiral magnet are hence no longer the conventional s ...

2021

Direct measurement of the triple spin flip rate in dynamic nuclear polarization

A previous study of the effect of Gadolinium doping on the dynamic polarization (DNP) of C-13 using trityls showed that the rate at which the polarization builds up is almost independent of the Gadolinium concentration, while the electron spin-lattice rela ...

2021

Methods to Enhance Nuclear Magnetic Resonance Sensitivity at High Magnetic Field

Claudia Christina Zanella

MR is a well-established technique routinely used in preclinical and clinical studies. This thesis focussed on the improvement of sensitivity of different methods in MR. Hyperpolarized 129Xe gas is used for studying pulmonary disease or cerebral perfusion ...

EPFL2021

In this thesis, we exploited optical and X-ray pump-probe methods in a synergistic approach to study the interplay of the electronic, spin and structural degrees of freedom in two class of complex systems relevant for solar energy conversion applications: ...

EPFL2021

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AMER CHEMICAL SOC2021

Endogenous O-17 Dynamic Nuclear Polarization of Gd-Doped CeO2 from 100 to 370 K

David Lyndon Emsley

Michael Allan Hope

Moreno Lelli

Snaedis Björgvinsdóttir

Georges Guévork Jean-Jacques Menzildjian

Bowen Zhang

Zhuoran Wang

Photo- and thermally-induced electronic and structural dynamics in perovskites and transition metal oxides

Oliviero Cannelli