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The redox chemistry of f-elements is drawing the attention of inorganic chemists due to their unusual reaction pathways. Notably low-valent f-element complexes have been shown to be able to activate small molecules such as CO2 and N2 in mild conditions. Co ...
Knowledge of fundamental chemical properties of all environmentally relevant uranium species is essential to understand environmental uranium mobility and develop novel remediation strate-gies. A myriad of uranium(VI) and uranium(IV) compounds has been stu ...
Aerosol-cloud interactions (ACI) constitute the single largest uncertainty in anthropogenic radiative forcing. To reduce the uncertainties and gain more confidence in the simulation of ACI, models need to be evaluated against observations, in particular ag ...
Here we report the effect of UO2+⋯Fe2+ cation–cation interactions on the redox properties of uranyl(V) complexes and on their stability with respect to proton induced disproportionation. The tripodal heptadentate Schiff base trensal3− ligand allowed the sy ...
Uranium (U) is a ubiquitous element in the Earth's crust at similar to 2 ppm. In anoxic environments, soluble hexavalent uranium (U(VI)) is reduced and immobilized. The underlying reduction mechanism is unknown but likely of critical importance to explain ...
Irradiation-induced segregation mechanisms are classified into solute-point-defect complex type and inverse Kirkendall type. For solutes that have a strong interaction with interstitials in a dilute alloy, the complex effect plays an important part in the ...
It has generally been assumed that the bioreduction of hexavalent uranium in groundwater systems will result in the precipitation of immobile uraninite (UO2). In order to explore the form and stability of uranium immobilized under these conditions, we intr ...
Neutron filters/attenuators have been designed and constructed as an upgrade of the JET gamma-ray cameras (GRC's). This diagnostics upgrade should reduce the neutron flux at the gamma-ray detectors in a way that it would make possible gamma-ray imaging mea ...
An integrated modelling methodology for the calculation of realistic plasma neutron sources for the JET tokamak has been developed. The computational chain comprises TRANSP plasma transport and DRESS neutron spectrum calculations, and their coupling to the ...
Segregation of P and Mo to prior austenite grain boundaries in a 2.25Cr1Mo steel subjected to neutron irradiation and ageing is examined using field emission gull scanning transmission electron microscopy (FEGSTEM) with energy dispersive X-ray microanalysi ...
