Concept

Femtochimie

Publications associées (102)

Experimental demonstration of attosecond pump-probe spectroscopy with an X-ray free-electron laser

Christoph Bostedt, Jun Wang, Zhaoheng Guo, Xiang Li, Siqi Li, Zhen Zhang

Pump-probe experiments with subfemtosecond resolution are the key to understanding electronic dynamics in quantum systems. Here we demonstrate the generation and control of subfemtosecond pulse pairs from a two-colour X-ray free-electron laser. By measurin ...

Nature Portfolio2024

Ultrafast Electron Microscopy of Nanoscale Charge Dynamics in Semiconductors

Fabrizio Carbone, Giovanni Maria Vanacore, Ivan Madan, Ido Kaminer, Simone Gargiulo, Francesco Barantani, Kangpeng Wang

The ultrafast dynamics of charge carriers in solids plays a pivotal role in emerging optoelectronics, photonics, energy harvesting, and quantum technology applications. However, the investigation and direct visualization of such nonequilibrium phenomena re ...

AMER CHEMICAL SOC2023

Terahertz waveform synthesis in integrated thin-film lithium niobate platform

Ileana-Cristina Benea-Chelmus, Jérôme Faist, Francesca Fabiana Settembrini

Bridging the "terahertz gap" relies upon synthesizing arbitrary waveforms in the terahertz domain enabling applications that require both narrow band sources for sensing and few-cycle drives for classical and quantum objects. However, realization of custom ...

Berlin2023

Tunable pump compression and fast modulation for pulsed THz generation

Ileana-Cristina Benea-Chelmus, Alessandro Tomasino, Yazan Lampert Almahmoud, Shima Rajabali

We demonstrate tunable dispersion compensation of femtosecond pulses at telecom wavelengths for broadband Terahertz generation in 7.5-meter fiber link using a Silicon prism pair. The prism pair enhances the amplitude of the THz E-field in InGaAs photocondu ...

New York2023

Analytics at the nanometer and nanosecond scales by short electron pulses in an electron microscope

Chemical reactions and phase transformations in nanometer-size objects may happen at very short timescales, so conventional characterization tools are not applicable. A new technique combining high spatial and temporal resolution is ultrafast (or dynamic) ...

SPRINGER2022

Optically Triggered Neel Vector Manipulation of a Metallic Antiferromagnet Mn2Au under Strain

Alexey Sapozhnik

The absence of stray fields, their insensitivity to external magnetic fields, and ultrafast dynamics make antiferromagnets promising candidates for active elements in spintronic devices. Here, we demonstrate manipulation of the Neel vector in the metallic ...

AMER CHEMICAL SOC2022

Spatio-Temporal Dynamics of Free and Bound Carriers in Photovoltaic Materials

Jacques-Edouard Moser, George Cameron Fish

Photoinduced charge separation into free carriers and subsequent charge transfer are key processes that govern the efficiencies of third generation solar cell technologies based on donor-acceptor heterojunctions. As these processes typically occur on picos ...

2022

Gain-switched semiconductor laser driven soliton microcombs

Tobias Kippenberg, Junqiu Liu, Erwan Guillaume Albert Lucas, Wenle Weng, Jijun He

Dissipative Kerr soliton generation using self-injection-locked III-V lasers has enabled fully integrated hybrid microcombs that operate in turnkey mode and can access microwave repetition rates. Yet, continuous-wave-driven soliton microcombs exhibit low e ...

NATURE RESEARCH2021

Broadband Quasi-Phase-Matching in All-Optically Poled Stoichiometric Silicon Nitride Waveguides

Camille Sophie Brès, Boris Zabelich, Edgars Nitiss

We show how broadband (>30nm) quasi-phase matching in all-optically poled Si3N4 waveguides provides a platform for efficient sum-frequency generation, and for femtosecond pulse processing such as fcEo detection without the need for group velocity engineeri ...

2020

Fundamentals and perspectives of ultrafast photoferroic recording

Anna Pogrebna

The ability to switch ferroics (ferro-, ferri-, antiferromagnets, ferroelectrics, multiferroics) between two stable bit states is one of the keystones of modern data storage technology. Due to many new ideas, originating from fundamental research during th ...

2020

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