Publications associées à Attosecond

Exciton migration in two-dimensional materials

Excitons play an essential role in the optical response of two-dimensional materials. These are bound states showing up in the band gaps of many-body systems and are conceived as quasiparticles formed by an electron and a hole. By performing real-time simu ...

Nature Portfolio2024

Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

Christoph Bostedt, Zhaoheng Guo, Jonas Knurr, Andre Al Haddad, Siqi Li

The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray t ...

ROYAL SOC CHEMISTRY2020

Spin polarization and attosecond time delay in photoemission from solids

Mauro Fanciulli

In the photoemission process electrons are emitted from a solid upon excitation with UV light. From the measurement of their energy and momentum, angle-resolved photoemission spectroscopy (ARPES) allows to reconstruct the electronic properties of the solid ...

EPFL2018

Auger-induced charge migration

Christoph Bostedt

Novel perspectives of controlling molecular systems have recently arisen from the possibility of generating attosecond pulses in the ultraviolet regime and tailoring electron dynamics in its natural time scale. The cornerstone mechanism is the so-called ch ...

2018

Charge migration and charge transfer in molecular systems

Majed Chergui, Ursula Röthlisberger, Jacques-Edouard Moser, Andrea Cannizzo, Natalie Renuka Banerji, Joël Teuscher, Christopher Alexander Arrell, Pablo Lopez Tarifa, Elisa Liberatore

The transfer of charge at the molecular level plays a fundamental role in many areas of chemistry, physics, biology and materials science. Today, more than 60 years after the seminal work of R. A. Marcus, charge transfer is still a very active field of res ...

2017

Spin Polarization and Attosecond Time Delay in Photoemission from Spin Degenerate States of Solids

Jan Hugo Dil, Stefan Peter Muff, Mauro Fanciulli

After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecond-resolved photoemission experiments. According to the Eisenbu ...

American Physical Society2017

Several Semiclassical Approaches to Time-resolved Spectroscopy

Jiri Vanicek

Ultrafast spectroscopy allows molecular dynamics to be resolved on the femtosecond time scale. Whereas such short time scales obviously pose any experimental challenges, they provide an opportunity for semiclassica methods, which are naturally suited for s ...

Swiss Chemical Soc2017

Laser arrival measurement tools for SwissFEL

Christoph Peter Hauri

SwissFEL is aiming to produce X-ray pulses from 30 fs down to the attosecond time scale. This requires the compression of the several picosecond long electron bunches produced by a photo-injector to sub-fs level. To achieve this, 40fs accurate injection of ...

Spie-Int Soc Optical Engineering2015

Picosecond solvation dynamics of alkali cations in superfluid 4He nanodroplets

Marcel Drabbels, Alberto Hernando de Castro

The dynamics following the photoionization of neutral Rb and Cs atoms residing in a dimple at the surface of a superfluid 4He1000 nanodroplet has been investigated within time-dependent density functional theory, complementing a previous study on Ba. The c ...

American Physical Society2014

Can Energetic Terahertz Pulses Initiate Surface Catalytic Reactions on the Picosecond Time Scale?

Christoph Peter Hauri

In preparation for picosecond pump-probe experiments at the SwissFEL X-ray laser facility, the feasibility of collectively initiating surface chemical reactions using energetic pulses of terahertz radiation is being tested. © Schweizerische Chemische Gesel ...

Schweizerische Chemische Gesellschaft2011