Majed Chergui

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Ultrafast X-ray Spectroscopy of Haem Proteins

Majed Chergui, Camila Bacellar Cases Da Silveira

In this article we revisit our recent picosecond and femtosecond X-ray absorption spectroscopy (XAS) and X-ray emission spectroscopy (XES) experiments, probing the ultrafast electronic and geometric evolution of photoexcited haem proteins, namely ferrous N ...

SWISS CHEMICAL SOC2022

Chiral control of spin-crossover dynamics in Fe (II) complexes

Majed Chergui, Malte Oppermann, Jérôme Lacour

Iron-based spin-crossover complexes hold tremendous promise as multifunctional switches in molecular devices. However, real-world technological applications require the excited high-spin state to be kinetically stable-a feature that has been achieved only ...

NATURE PORTFOLIO2022

Carbon K-edge x-ray emission spectroscopy of gas phase ethylenic molecules

Majed Chergui, Camila Bacellar Cases Da Silveira, Rebecca Ann Ingle, Luca Longetti, Thomas Roland Barillot

We report on the C K-edge x-ray absorption spectra and the resonant (RXES) and non-resonant (NXES) x-ray emission spectra of ethylene, allene and butadiene in the gas phase. The RXES and NXES show clear differences for the different molecules. Overall both ...

IOP Publishing2022

Optically induced changes in the band structure of the Weyl charge-density-wave compound (TaSe4)(2)I

Majed Chergui, Marco Grioni, Oleg Yazyev, Daniel Gosalbez Martinez, Michele Puppin, Helmuth Berger, Alberto Crepaldi

Collective modes are responsible for the emergence of novel quantum phases in topological materials. In the quasi-one dimensional (1D) Weyl semimetal (TaSe4)(2)I < i , a charge density wave (CDW) opens band gaps at the Weyl points, thus turning the system ...

2022

Quantifying Photoinduced Polaronic Distortions in Inorganic Lead Halide Perovskite Nanocrystals

Majed Chergui, Nicola Colonna, Michele Puppin, Giulia Fulvia Mancini, Thomas Charles Henry Rossi, Andre Al Haddad, Dominik Kinschel, Oliviero Cannelli, James Michael Budarz, Ludmila Maria Diniz Leroy

The development of next-generation perovskite-based optoelectronic devices relies critically on the understanding of the interaction between charge carriers and the polar lattice in out-of-equilibrium conditions. While it has become increasingly evident fo ...

2021

Hard X-ray transient grating spectroscopy on bismuth germanate

Majed Chergui, Giulia Fulvia Mancini, Jérémy Raymond Jean Maurice Rouxel

Optical-domain transient grating (TG) spectroscopy is a versatile background-free four-wave-mixing technique that is used to probe vibrational, magnetic and electronic degrees of freedom in the time domain(1). The newly developed coherent X-ray free-electr ...

Nature Publishing Group2021

Femtosecond X-ray spectroscopy of haem proteins

Majed Chergui, Giulia Fulvia Mancini, Camila Bacellar Cases Da Silveira, Dominik Kinschel, Oliviero Cannelli, Boris Sorokin

We discuss our recently reported femtosecond (fs) X-ray emission spectroscopy results on the ligand dissociation and recombination in nitrosylmyoglobin (MbNO) in the context of previous studies on ferrous haem proteins. We also present a preliminary accoun ...

ROYAL SOC CHEMISTRY2021

Mapping the thermo-induced valence tautomerism in Cobalt dioxolane single crystals

Majed Chergui, Frederico Alves Lima, Ludmila Maria Diniz Leroy

INT UNION CRYSTALLOGRAPHY2021

Broadband visible two-dimensional spectroscopy of molecular dyes

Majed Chergui, Andre Al Haddad, Lars-Hendrik Mewes, Rebecca Ann Ingle

Two-dimensional Fourier transform spectroscopy is a promising technique to study ultrafast molecular dynamics. Similar to transient absorption spectroscopy, a more complete picture of the dynamics requires broadband laser pulses to observe transient change ...

AMER INST PHYSICS2021

Strain wave pathway to semiconductor-to-metal transition revealed by time-resolved X-ray powder diffraction

Majed Chergui, Giulia Fulvia Mancini

One of the main challenges in ultrafast material science is to trigger phase transitions with short pulses of light. Here we show how strain waves, launched by electronic and structural precursor phenomena, determine a coherent macroscopic transformation p ...

Nature Research2021

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