Publications de Jie Zhang | EPFL Graph Search

Cooperative promotion of electroreduction of CO to n-propanol by *CO enrichment and proton regulation

The CO2/CO electroreduction reaction (CO2RR/CORR) to liquid products presents an enticing pathway to store intermittent renewable electricity. However, the selectivity for desirable high-value C3 products, such as n-propanol, remains unsatisfactory in the ...

ROYAL SOC CHEMISTRY2025

Scalable synthesis of Cu-cluster catalysts via spark ablation for the electrochemical conversion of CO 2 to acetaldehyde

Cedric David Koolen, Wen Luo, Jie Zhang, Mo Li, Olga Safonova

The electrochemical conversion of CO 2 into acetaldehyde offers a sustainable and green alternative to the Wacker process. However, current electrocatalysts cannot effectively compete with heterogeneous processes owing to their limited selectivity towards ...

Springer Science and Business Media LLC2025

Selective electroreduction of CO2 to C2+ products on cobalt decorated copper catalysts

Andreas Züttel, Jie Zhang, Kun Zhao

Cu-catalyzed electrochemical CO2 reduction reaction (CO2RR) to multi-carbon (C2+) products is often plagued by low selectivity because the adsorption energies of different reaction intermediates are in a linear scaling relationship. Development of Cu-based ...

2024

Low-temperature non-equilibrium synthesis of anisotropic multimetallic nanosurface alloys for electrochemical CO2 reduction

Andreas Züttel, Emad Oveisi, Cedric David Koolen, Jie Zhang, Mo Li

Multimetallic nanoparticles are of interest as functional materials due to their highly tunable properties. However, synthesizing congruent mixtures of immiscible components is limited by the need for high-temperature procedures followed by rapid quenching ...

Springernature2023

Tandem effect of Ag@C@Cu catalysts enhances ethanol selectivity for electrochemical CO2 reduction in flow reactors

Andreas Züttel, Thi Ha My Pham, Cedric David Koolen, Wen Luo, Jie Zhang, Mo Li, Youngdon Ko, Liping Zhong

CO-selective metals (e.g., Ag) on Cu catalysts improve the selec-tivity of multi-carbon (C2+) products in electrochemical CO2 reduc-tion. However, the origin of the improvement remains unclear due to the convolution of tandem and interface effects. Here, A ...

ELSEVIER2022

Active sites on copper-based catalysts for electrochemical CO2 reduction selectively to C2+ products

Jie Zhang

Electrochemical CO2 reduction (eCO2RR) towards value-added chemicals, powered by renewable electricity, is a promising technology for storing the intermittent renewable energy in the form of chemical bonds. Among the various products of eCO2RR, multi-carbo ...

EPFL2022

Electrospun nanofibers for electrochemical reduction of CO2: A mini review

Andreas Züttel, Wen Luo, Jie Zhang

The electrochemical reduction of CO2 (CO2RR) into valuable products represents a step towards alleviating global warming and the energy crisis. However, the sluggish kinetics of the CO2RR and the competitive hydrogen evolution reaction (HER) still limit th ...

Elsevier2021

Hydrogen Storage by Reduction of CO2 to Synthetic Hydrocarbons

Andreas Züttel, Noris André Gallandat, Wen Luo, Jie Zhang, Kun Zhao

The storage of renewable energy is crucial for the substitution of fossil fuels with renewable energy. Hydrogen is the first step in the conversion of electricity from renewable sources to an energy carrier. However, hydrogen is technically and economicall ...

2021

Electrochemical reconstruction of ZnO for selective reduction of CO2 to CO

Andreas Züttel, Emanuele Moioli, Wen Luo, Kun Zhao, Jie Zhang, Qin Zhang

Electrocatalytic conversion of CO2 to valuable chemicals is a highly promising route to close the carbon cycle. Herein, Zn catalysts derived from electrochemical reconstruction of ZnO materials are presented as efficient CO2-to-CO catalysts. We found that ...

2020

A metal-organic framework/polymer derived catalyst containing single-atom nickel species for electrocatalysis

Wendy Lee Queen, Emad Oveisi, Wen Luo, Daniel Teav Sun, Shuliang Yang, Li Peng, Jie Zhang, Mehrdad Asgari, Olga Trukhina, Dragos-Constantin Stoian

While metal-organic frameworks (MOF) alone offer a wide range of structural tunability, the formation of composites, through the introduction of other non-native species, like polymers, can further broaden their structure/property spectrum. Here we demonst ...

2020