Tunable Metal Oxide Shell as a Spacer to Study Energy Transfer in Semiconductor Nanocrystals

Publications associées (21)

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Highly soluble energy relay dyes for dye-sensitized solar cells

Michael Graetzel, Jun Ho Yum

High solubility is a requirement for energy relay dyes (ERDs) to absorb a large portion of incident light and significantly improve the efficiency of dye-sensitized solar cells (DSSCs). Two benzonitrile-soluble ERDs, BL302 and BL315, were synthesized, char ...

Royal Society of Chemistry2013

Long-distance radiative excitation transfer between quantum dots in disordered photonic crystal waveguides

Vincenzo Savona, Momchil Minkov

We theoretically investigate the magnitude and range of the photon-mediated interaction between two quantum dots embedded in a photonic crystal waveguide, including fabrication disorder both in the crystal and in the dot positioning. We find that disorder- ...

Amer Physical Soc2013

Enhancing the efficiency of a dye sensitized solar cell due to the energy transfer between CdSe quantum dots and a designed squaraine dye

Michael Graetzel, Mohammad Khaja Nazeeruddin, Lioz Etgar, Guido Viscardi

The power conversion efficiency of a dye-sensitized solar cell with tailored squaraine dye enhanced by 47%, due to Forster resonance energy transfer from CdSe quantum dots to the squaraine dye. The incident photons to collection efficiency of electrons ind ...

2012

Linear and Time-Resolved THz Spectroscopy of Photonic and Charge Transporting Systems

Jan Cornelius Brauer

Photo-induced charge separation and charge transport are fundamental processes in many energy conversion techniques, where light is converted into chemical energy (PEC), into electrical energy (solar cells) or in the opposite sense if electrical energy is ...

EPFL2012

On the Morphology and Interfaces of Nanostructured Hematite Photoanodes for Solar-Driven Water Splitting

Florian Le Formal

A sustainable route to store the energy provided by the Sun, is to directly convert sunlight into molecular hydrogen using a semiconductor performing water photolysis. Hematite (α-Fe2O3) is promising for this application due to its ample abundance, chemica ...

EPFL2011

Ultrafast Visible and Ultraviolet Fluorescence Studies of Molecular and Biological Sytems in Solution

Olivier Christian Bräm

A wide variety of physical and chemical processes at the molecular level, as charge or energy transfer, solvation, electronic as well as vibrational relaxation, is at the origin of the biological functionality of proteins. The work reported in this thesis ...

EPFL2011

Photoelectrochemical Water Splitting with Mesoporous Hematite Prepared by a Solution-Based Colloidal Approach

Michael Graetzel, Kevin Sivula, Florian Le Formal

Sustainable hydrogen production through photoelectrochemical water splitting using hematite (alpha-Fe2O3) is a promising approach for the chemical storage of solar energy, but is complicated by the material's nonoptimal optoelectronic properties. Nanostruc ...

American Chemical Society2010

Phosphorescent energy relay dye for improved light harvesting response in liquid dye-sensitized solar cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Jun Ho Yum

Energy transfer from phosphorescent ruthenium complex N877 dissolved in the liquid electrolyte to the squaraine sensitizer SQ1 anchored on the titanium oxide surface resulted in a four fold increase in external quantum efficiency in the blue part of the vi ...

Royal Society of Chemistry2010

Photoelectrochemical properties of sensitized thin films

Mohamad Hojeij

In recent years, the fabrication of novel ultrathin film systems featuring multi-functionalities has been extensively studied due to their potential applications in photonics, sensors and solar cells. In a general sense, the primary goal of the present the ...

EPFL2009

Sub-picosecond polychromatic photoluminescence studies of CdSe and PbSe nanodots

Majed Chergui, Frank van Mourik, Andrea Cannizzo, Camilla Bonati

We present our studies of femtosecond photoluminescence of colloidal solns. of CdSe and PbSe nanocrystals, using polychromatic fluorescence upconversion. Ultrafast relaxation processes are obsd. in both cases upon excitation at 400 nm and 800 nm resp. Unde ...

2008

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Enhancing the efficiency of a dye sensitized solar cell due to the energy transfer between CdSe quantum dots and a designed squaraine dye

Michael Graetzel, Mohammad Khaja Nazeeruddin, Lioz Etgar, Guido Viscardi

2012