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This thesis works reports on the magnetic properties of single transition metal atoms and hydrogenated compounds adsorbed on crystal surfaces. It is an experimental study, based on scanning tunneling microscopy (STM), initiated by the project of demonstrat ...
Multiscale coupling of a quantum mechanical (QM) domain to a coarser-scale material description in a larger surrounding domain should yield forces and energies in the QM domain that are the same as would be achieved in a QM simulation of the entire system. ...
Muon spin resonance (mu SR) is a powerful technique for investigating the local magnetic fields in materials through implanted muons. Here we report a mu SR study of chemically produced thermally exfoliated graphene. Our results provide an experimental ans ...
Millimeter-sized cobalt doped rutile crystals with a bi-pyramidal shape are obtained by chemical vapour transport using scroll-type H2Ti3O7 nanotubes as a precursor in which Co2+ ions are introduced by a simple ion exchange method prior to the growth. Desp ...
We investigate the temperature dependence of the Yb valence in YbMn6Ge1.8Sn4.2 and YbMn6Ge1.6Sn4.4 using resonant inelastic x-ray scattering experiments. Yb is found to be in an intermediate valent state in the whole investigated temperature range (10-450 ...
The edges of graphene nanoribbons (GNRs) have attracted much interest due to their potentially strong influence on GNR electronic and magnetic properties. Here we report the ability to engineer the microscopic edge termination of high-quality GNRs via hydr ...
Magnetic properties of a large assembly of ultrathin graphitic particles obtained by heavy sonication of graphite powder dispersed in N-methylpyrrolidone were measured by electron-spin resonance (ESR). The ESR signal was decomposed into one narrow and one ...
Gd3N@C-80 endohedral fullerene, a starting material for a potential magnetic resonance imaging contrast agent, is investigated by high-frequency electron spin resonance (ESR) and SQUID magnetometry. The magnetic moments of the three Gd ions of the endohedr ...
Novel magnetic materials are constantly emerging. This thesis reports an Electron Spin Resonance (ESR) study on three novel materials of great scientific interest: monoclinic SeCuO3 compound representing a network of tetramers, large assembly of ultrathin ...
The olivine compound Mn2GeO4 is shown to feature both a ferroelectric polarization and a ferromagnetic magnetization that are directly coupled and point along the same direction. We show that a spin spiral generates ferroelectricity, and a canted commensur ...