Trace gas and aerosol interactions in the fully coupled model of aerosol-chemistry-climate ECHAM5-HAMMOZ: 2. Impact of heterogeneous chemistry on the global aerosol distributions
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Particle acidity affects aerosol concentrations, chemical composition and toxicity. Sulfate is often the main acid component of aerosols, and largely determines the acidity of fine particles under 2.5 μm in diameter, PM2.5. Over the past 15 years, atmosphe ...
Aerosol iron was examined in Saharan dust plumes using a combination of iron near-edge X-ray absorption spectroscopy and wet-chemical techniques. Aerosol samples were collected at three sites located in the Mediterranean, the Atlantic, and Bermuda to chara ...
Fundamental questions remain about the origin of newly formed atmospheric aerosol particles because data from laboratory measurements have been insufficient to build global models. In contrast, gas-phase chemistry models have been based on laboratory kinet ...
American Association for the Advancement of Science2016
We investigate the effects of anthropogenic sulfate on secondary organic aerosol (SOA) formation from biogenic isoprene through airborne measurements in the southeastern United States as part of the Southeast Nexus (SENEX) field campaign. In a flight over ...
Our understanding of the interactions of aerosols and clouds has a strong heritage in laboratory experiments, field measurements, and process modeling. We present a review on the state of knowledge for mineral dust emitted from major global dust source reg ...
We introduce a framework to efficiently parameterise the aerosol water uptake for mixtures of semi-volatile and non-volatile compounds, based on the coefficient, vi. This solute-specific coefficient was introduced in Metzger et al. (2012) to accurately par ...
Biogenic influences on the composition and characteristics of aerosol were investigated on Bird Island (54°00' S, 38°03' W) in the South Atlantic during November and December 2010. This remote marine environment is characterised by large seabird and seal c ...
As human impact have been increasing strongly over the last decades, it is crucial to distinguish human-induced dust sources from natural ones in order to define the boundary of a newly proposed epoch -the Anthropocene. Here, we track anthropogenic signatu ...
This work estimates the primary marine organic aerosol global emission source and its impact on cloud condensation nuclei (CCN) concentrations by implementing an organic sea spray source function into a series of global aerosol simulations. The source func ...
The US Environmental Protection Agency's (EPA) Community Multiscale Air Quality (CMAQ) modeling system version 4.7 is further developed to enhance its capability in simulating the photochemical cycles in the presence of dust particles. The new model treatm ...