An investigation of laser intensity and temperature effects in the time-resolved infrared multiphoton dissociation of chlorodifluoromethane
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The equil. I2(g) + 2NO(g) = 2INO(g) was studied at room temp. by UV absorption spectroscopy. The equil. const. was measured as kp = (2.7 +- 0.3) * 10-6 atm-1 at 298 K. The 3rd-law calcns. lead to DHf(INO) of 120.0 +- 0.3 kJ/mol. The relative absorption spe ...
The temp. jump relaxation method was used for kinetic measurements in the gas phase. The system N2O4 .dblarw. 2NO2 was studied. Fast temp. jumps were induced by IR absorption from a CO2 laser. Temp. jumps of
The IR multiphonon dissocn. of CF2HCl was investigated by monitoring the appearance of the CF2 product in real time during and after the laser pulse. The difluorcarbene radicals were detected quant. by their optical absorption in the ~A1B1->~X1A1 band syst ...
