Surface-Plasmon-Induced Modification on the Spontaneous Emission Spectrum via Subwavelength-Confined Anisotropic Purcell Factor
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Intensive developments of plasmonic nanomaterials over recent decades have inspired appealing applications in biosensing, optical trapping, fluorescence enhancement and light harvesting in solar cells. These nanostructures supporting unique light-matter in ...
EPFL2017
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The interaction between 3, 4, 9, 10-perylenetetracarboxylic dianhydride (PTCDA) molecules and solid rare gas samples is studied by means of fluorescence emission spectroscopy. Laser-excited PTCDA-doped large argon, neon, and para-hydrogen clusters along wi ...
In 1906, Theodore Lyman discovered his eponymous series of transitions in the extreme-ultraviolet region of the atomic hydrogen spectrum(1,2). The patterns in the hydrogen spectrum helped to establish the emerging theory of quantum mechanics, which we now ...
Photonic crystal (PhC) cavities combine ultra-high quality (Q) factors with small mode volumes, resulting in an enhancement of the light-matter interaction at the nanoscale, which, beyond fundamental studies is advantageous for countless applications in ph ...
Drexhage’s seminal observation that spontaneous emission rates of fluorophores vary with distance from a mirror uncovered the fundamental notion that a source’s environment determines radiative linewidths and shifts. Further, this observation established a ...
The properties of semiconductors heterostructures of nanoscopic dimensions change from that of bulk material according to the rules of quantum mechanics. The planar quantum wells (QWs) are widely used in various diode and laser devices thanks to the relati ...
The most widely used substrates for fluorescent immunoassay are based on transparent materials such as glass or plastic with almost no optical functionality. Very recently, optical nanostructures made of metal on dielectrics have been proposed to perform p ...
This thesis works reports on the magnetic properties of single transition metal atoms and hydrogenated compounds adsorbed on crystal surfaces. It is an experimental study, based on scanning tunneling microscopy (STM), initiated by the project of demonstrat ...
EPFL2013
Optical frequency references are devices providing well-defined and stable optical frequency responses to incoming radiation for applications such as high-precision spectroscopy and optical fibre communications. To stabilise the emission frequency of laser ...
EPFL2012
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We investigate the mediation of symmetry-forbidden atomic transitions using plasmonic nanostructures. We show that the excitation of the electric dipole-forbidden, quadrupole-allowed 6 2S1/2 − 5 2D5/2 transition in cesium may be enhanced by more than 6 ord ...
