Electronic and magnetic properties of bulk Cr tips for scanning tunneling spectroscopy
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This thesis presents a combined experimental and theoretical study of the classical and quantum magnetization dynamics in single magnetic adatoms and molecules, and on the classical and quantum coherent control thereof. First, a detailed description of the ...
EPFL2021
This thesis investigates the magnetic properties of single atoms and dimers adsorbed on graphene and oxide decoupling layers supported by single crystal metal substrates, using scanning tunneling microscopy (STM) and spin-polarized scanning tunneling micro ...
EPFL2022
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The Josephson effect in scanning tunneling microscopy (STM) is an excellent tool to probe the properties of a superconductor on a local scale. We use atomic manipulation in a low temperature STM to create mesoscopic single channel contacts and study the Jo ...
The magnetic properties and the atomic scale morphology of bimetallic two-dimensional nanoislands, epitaxially grown on fcc(111) metal surfaces, have been studied by means of Magneto-Optical Kerr Effect and Scanning Tunneling Microscopy. We investigate the ...
The low-energy electronic structure of nanographenes can be tuned through zero-energy pi-electron states, typically referred to as zero-modes. Customizable electronic and magnetic structures have been engineered by coupling zero-modes through exchange and ...
We report on scanningtunneling microscopy (STM) topographs ofindividual metal phthalocyanines (MPc) on a thin salt (NaCl) filmadsorbed on a gold substrate, at tunneling energies within the molecule'selectronic transport gap. Theoretical models of increasin ...
The magnetic force microscope (MFM) is an established experimental tool for imaging stray fields with high spatial resolution and sensitivity. The MFM contrast can however contain contributions from the sample topography, variations in the surface Kelvin p ...
Tracking electron motion in molecules is the key to understanding and controlling chemical transformations. Contemporary techniques in attosecond science are able to generate and trace the consequences of this motion in real time, but not in real space. Sc ...
Spin-dependent scattering from magnetic impurities inside a superconductor gives rise to Yu-Shiba-Rusinov (YSR) states within the superconducting gap. They can be modeled by the largely equivalent Kondo or Anderson impurity models. The role of the magnetic ...
Unification of the techniques of ultrafast science and scanning tunneling microscopy (STM) has the potential of tracking electronic motion in molecules simultaneously in real space and real time. Laser pulses can couple to an STM junction either in the wea ...