Optical label-free and model-free probe of the surface potential of nanoscale and microscopic objects in aqueous solution
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This thesis explores transport phenomena in nanochannels on a chip. Fundamental nanofluidic ionic studies form the basis for novel separation and preconcentration applications for proteomic purposes. The measurements were performed with 50-nm-high 1D nanoc ...
Organisation and heterogeneous photoreactivity of water-soluble zinc meso-tetrakis(4-carboxyphenyl) porphyrin (ZnTPPC) were investigated at polarisable liquid / liquid interfaces by systematically varying the organic phase solvent. The remarkable affinity ...
The interface between two immiscible electrolyte solutions (ITIES), or liquid|liquid interface, provides a defect-free junction for fundamental studies of adsorption phenomena, heterogeneous charge transfer reactions, and phase-formation processes. Recent ...
This dissertation addresses the adsorption of proteins in microchannels with the aim of improving the result of an immunoassay. To observe the adsorption of fluorescently labelled immunoglobulins G in laser ablated polymer microchannels, a confocal microsc ...
Monolayer adsorption of benzoic acid derivatives on activated oxide surfaces from solution and from the vapor phase are investigated with the view of modifying the work function of a conductive substrate. Para-substituted benzoic acids with a wide range of ...
This paper presents an original semi-analytical method (SAM) for computing the 2-D current distribution in conductors and superconductors of arbitrary shape, discretized in triangular elements. The method is a generalization of the one introduced by Brandt ...
Adsorption of charged species at the interface between two immiscible electrolyte solutions (ITIES) is simulated taking into account both the mutual influence between the potential dependent surface excess charge and the potential distribution between the ...
The voltage induced assembly and photoreactivity of cadmium selenide (CdSe) nanoparticles protected by mercaptosuccinic acid are studied at the polarisable interface between water and 1,2-dichloroethane electrolyte solutions. Cyclic voltammograms and admit ...
The adsorption of ions at the interface between two immiscible electrolyte solutions (ITIES) is primarily controlled by the potential distribution across the interface, which in turn is influenced by the adsorption process. In the present paper, we simulat ...
The present invention provides methods and apparatus for locally patterning surfaces. In one such method, an oxidizable thioether is adsorbed onto a conductive surface 10. The surface is then contacted with a fluid medium M. A conducting stamp 12 is then b ...
