Four new noncentrosymmetric salt-inclusion vanadates: (AX)2Mn(VO3)2 (A/X = Rb/Cl, Cs/Cl, Cs/Br) and (CsCl)2Cu(VO3)2
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In conventional homogeneous catalysis, supporting ligands act as spectators that do not interact directly with substrates. However, in metal–ligand cooperative catalysis, ligands are involved in facilitating reaction pathways that would be less favourable ...
Owing to the almost boundless structural tunability, MOF and MOF‐derived catalysts have recently exhibited structures of higher complexity, and hence, have demonstrated activity in a wide array of organic transformations. These reactions have a broad range ...
The industrial production of aromatic amines, essential intermediates for the synthesis of several drugs, dyes, pigments and agrochemicals, requires the use of heterogeneous catalysis. These molecules were formerly produced by the Béchamp reduction, a non- ...
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The main aim of this dissertation is to study the catalytic aspects of very small transition metal clusters supported on h-BN/Rh(111). The catalytic reactions of interest were ammonia synthesis and CO oxidation on mass selected and soft landed iron and pla ...
Accurately simulating heterogeneously catalyzed reactions requires reliable barriers for molecules reacting at defects on metal surfaces, such as steps. However, first- principles methods capable of computing these barriers to chemical accuracy have yet to ...
In conventional homogeneous catalysis, supporting ligands act as spectators that do not interact directly with substrates. However, in metal–ligand cooperative catalysis, ligands are involved in facilitating reaction pathways that would be less favourable ...
Continuous catalytic supercritical water gasification (CSCWG; 400 degrees C, 28 MPa) of microalgal biomass (Chlorella vulgaris) was carried out at the microalgae production site of ZHAW in Wadenswil (Switzerland) non-stop over a period of 100 h. Characteri ...
Transition-metal-catalyzed hydrosilylation of olefins is one of the most important methods for the preparation of organosilicon compounds, which have broad applications in both synthetic and material chemistry. For decades, precious metals, principally pla ...
