Relationship between structures and activities of supported metal vanadates for the selective catalytic reduction of NO by NH3
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Under periodic lean/rich operation generated by repeated O2 pulses (O2-dithering), the abatement of CH4 and NO is enhanced compared to static operation. However, it is not well understood how the dithering parameters (pulse amplitude and frequency) affect ...
Iron-exchanged zeolites are industrial heterogeneous catalysts deployed to remediate anthropogenic emissions of both nitrous oxide (N2O) and nitrogen oxides (NOx = NO + NO2). Despite the extensive scientific attention received, limited knowledge is availab ...
Monomeric Fe species in zeolites are considered to be the active sites for the low temperature activity toward ammonia-assisted selective catalytic reduction of nitrogen oxides (NH3-SCR) in exhaust gases. Herein, we report on a preparation method to synthe ...
Natural gas (NG) is a suitable alternative to gasoline and diesel fuels to decrease the carbon footprint of the mobility and energy sectors. Although NG is considered a fossil fuel, methane (CH4), its main component, can be produced industrially from power ...
The effect of water on the NH3-assisted selective catalytic reduction of NOx (NH3-SCR) has been largely neglected, despite the inevitable presence of water vapor in real emissions produced by fuel combustion. In this work, we investigated the role of water ...
Cu-exchanged small-pore SSZ-13 catalysts have found wide use for the selective catalytic reduction (SCR) of nitrogen oxides from automotive exhaust gases. The transient working environment of the Cu-SSZ-13 catalyst during NH3-SCR requires studying the rate ...
The tightening emission regulations have led to the development of commercial DOCs with zoned or layered formulations allowing to cover a wide range of functionalities (i.e. CO, HC and NO oxidation as well as HC or NOx trap). Aging phenomena in such comple ...
Understanding the mechanisms behind chemical transformations is key to developing improved catalytic systems. To this end, operando spectroscopy has contributed significantly to the advancement of our molecular view of many reactions at the heart of the ch ...
Rhodium nanoparticles embedded on the interior of hollow porous carbon nanospheres, able to sieve monomers from polymers, were used to confirm the precise role of metal catalysts in the reductive catalytic fractionation of lignin. The study provides clear ...
Platinum (Pt) is a key material in automotive catalytic converters used to clean up the exhaust of the combustion engine. Pt particles in a ceramic matrix serve as an oxidation catalyst to eliminate toxic carbon monoxide (CO) and unburned hydrocarbons (CxH ...
