Suppression in droplet growth kinetics by the addition of organics to sulfate particles
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Ammonium sulfate particles were generated by atomization and introduced into a smog chamber where they were coated with secondary organic aerosol from ozonolysis of limonene or alpha-pinene. These mixed particles were then sampled with a humidified Tandem- ...
This study focuses on the importance of solute dissolution kinetics for cloud droplet formation. To comprehensively account for the kinetics, a numerical model of the process was developed. Simulations of cloud droplet growth were performed for solute diff ...
The performance of microfabricated piezoresistive cantilever array sensors has been evaluated using various vapors of volatile organic compounds including alkanes with different chain length from 5 (n-pentane) to 14 (n-tetradecane). We demonstrate that pie ...
Contact freezing of single supercooled water droplets colliding with kaolinite dust particles has been investigated. The experiments were performed with droplets levitated in an electrodynamic balance at temperatures from 240 to 268 K. Under relatively dry ...
Measurements of cloud condensation nuclei (CCN) concentrations (cm -3) between 0.2 and 1.0% supersaturation, aerosol size distribution and chemical composition were performed at a remote marine site in the eastern Mediterranean, from September to October 2 ...
This study investigates the droplet formation characteristics of secondary organic aerosol (SOA) formed during the ozonolysis of sesquiterpene β-caryophyllene (with and without hydroxyl radicals present). Emphasis is placed on understanding the role of sem ...
The ability of secondary organic aerosol (SOA) produced from the ozonolysis of α-pinene and monoterpene mixtures (α-pinene, β-pinene, limonene and 3-carene) to become cloud droplets was investigated. A static CCN counter and a Scanning Mobility CCN Analyse ...
Dust and black carbon aerosol have long been known to exert potentially important and diverse impacts on cloud droplet formation. Most studies to date focus on the soluble fraction of these particles, and overlook interactions of the insoluble fraction wit ...
This work offers for the first time a comprehensive parameterization suitable for large-scale models which is robust, computationally efficient, and from first principles links chemical effects, aerosol heterogeneity and entrainment with cloud droplet form ...
This study analyzes 27 cumuliform and stratiform clouds sampled aboard the CIRPAS Twin Otter during the 2004 International Consortium for Atmospheric Research on Transport and Transformation (ICARTT) experiment. The data set was used to assess cloud drople ...