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CONSPECTUS: The properties of transition metal complexes are interesting not only for their potential applications in solar energy conversion, OLEDs, molecular electronics, biology, photochemistry, etc. but also for their fascinating photophysical properti ...
Combining photoemission spectroscopy, Raman spectroscopy, and first-principles calculations, we characterize superconducting TlNi2Se2 as a material with weak electronic Coulomb correlations leading to a bandwidth renormalization of 1.4. We identify a camel ...
The first section of the thesis discusses the development and implementation of a two dimensional Fourier transform spectroscopy setup, that permits the recording of electronic 2D spectra in the visible regime. A hollow core fiber was used to generate broa ...
Today's brightest coherent X-ray sources, X-ray free-electron lasers, produce ultrafast X-ray pulses for which full-width at half-maximum durations as short as 3 fs have been measured(1). There has been a marked increase in the popularity of such short pul ...
We present a simple electron time of flight spectrometer for time resolved photoelectron spectroscopy of liquid samples using a vacuum ultraviolet (VUV) source produced by high-harmonic generation. The field free spectrometer coupled with the time-preservi ...
Multi-dimensional spectroscopies with vacuum ultraviolet (VUV)/x-ray free-electron laser (FEL) sources would open up unique capabilities for dynamic studies of matter at the femtosecond-nanometer time-length scales. Using sequences of ultrafast VUV/x-ray p ...
Institute of Physics (IoP) and Deutsche Physikalische Gesellschaft2013
Capturing the evolving geometric and electronic structure in the course of a chemical reaction or biological process is the principal aim of time-resolved X-ray spectroscopies. Recent technological and methodological improvements, such as high repetition r ...
Recently, much attention has been devoted to the development of new pulsed sources of radiation for investigating matter with atomic scale temporal and spatial resolution. While much has been achieved thanks to modern ultrafast laser technology, the ultima ...
Recent advances in ultrafast technology enable both the study and the control of materials properties thanks to the ability to record high temporal resolution movies of their transformations, or the ability to generate new states of matter by selecting ad ...
Determining the conformation of biological molecules is key for understanding their function. The recent combination of mass spectrometry, cryogenic ion traps, and laser spectroscopy is providing new methods to interrogate individual conformations of pepti ...
