TinyPols: a family of water-soluble binitroxides tailored for dynamic nuclear polarization enhanced NMR spectroscopy at 18.8 and 21.1 T
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A novel ligand, H12L, based on a trimethylbenzene core bearing three methylenediethylenetriamine-N,N,N,N- tetraacetate moieties (–CH2DTTA4–) for Gd3+ chelation has been synthesized, and its trinuclear Gd3+ complex [Gd3L(H2O) 6]3– investigated with respect ...
Scanning probe microscopy has become, nowadays, a branch of microscopy widely used to image surfaces of different specimens. Among the various applications, the magnetic imaging is one of the most exciting scanning probe microscopy techniques. It allows th ...
The excitation spectrum of a model magnetic system, LiHoF4, was studied with the use of neutron spectroscopy as the system was tuned to its quantum critical point by an applied magnetic field. The electronic mode softening expected for a quantum phase tran ...
This method measures cross relaxation rates in highly resolving NMR spectroscopy, where the sample substance is dissolved in a liq. and has nuclei A and X which have different chem. shifts WA and WX in a homogeneous static magnetic field Bo in the directio ...
The magnetic resonance at 41 meV observed in neutron scattering studies of YBa2Cu3O7 holds a key position in the understanding of high-T-c, superconductivity. Within the SO(5) model for superconductivity and antiferromagnetism, we have calculated the effec ...
In a method for exciting transverse magnetization by irradiating a nuclear spin system subjected to a const. magnetic field with a frequency-modulated RF-pulse (chirp-pulse) and with a further frequency-modulated RF-pulse (further chirp-pulse) for refocusi ...
Microfabricated probes for Nuclear Magnetic Resonance (NMR) spectroscopy of living cells in very small quantities have been developed in this thesis. These microprobes are based on two different sample interfaces: Channel microprobes, which confine a stack ...
The current approaches used for the analysis of electron paramagnetic resonance spectra of Gd3+ complexes suffer from a number of drawbacks. Even the elaborate model of [Rast et al., J. Chem. Phys. 113, 8724 (2000)] where the electron spin relaxation is ex ...
The transition metal tellurium oxychloride, Ni-5(TeO3)(4)Cl-2, has been investigated by high-field electron-spin resonance for frequencies up to 3 THz, at temperatures well below the magnetic ordering at 23 K. At zero external field several resonance modes ...
The water-soluble endohedral gadofullerene derivatives, Gd@C60(OH)x and Gd@C60[C(COOH)2]10, have been characterized with regard to their MRI contrast agent properties. Water-proton relaxivities have been measured in aqueous solution at variable temperature ...
