Electronic Population Transfer via Impulsive Stimulated X-Ray Raman Scattering with Attosecond Soft-X-Ray Pulses
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We describe a complete technological system at Imperial College London for Attosecond Science studies. The system comprises a few-cycle, carrier envelope phase stabilized laser source which delivers sub 4 fs pulses to a vibration-isolated attosecond vacuum ...
In the 60's, control, signals and systems had a common linear algebraic background and, according to their evolution, their respective backgrounds have now dramatically differed. Recovering such a common background, especially in the nonlinear context, is ...
A wide variety of physical and chemical processes at the molecular level, as charge or energy transfer, solvation, electronic as well as vibrational relaxation, is at the origin of the biological functionality of proteins. The work reported in this thesis ...
Time-resolved photoelectron spectroscopy can obtain detailed information about the dynamics of a chemical process on the femtosecond timescale. The resulting signal from such detailed experiments is often difficult to analyze and therefore theoretical calc ...
Solvation dynamics, the process of solvent reorganization upon electronic excitation of a solute, is central to our understanding chemical reactions in liquid phase. Ultrafast optical studies of solvation dynamics have so far been carried out on polyatomic ...
Electron beams in modern linear accelerators are now becoming limited in brightness by the intrinsic emittance of the photocathode electron source. Therefore it becomes important for large scale facilities such as free electron lasers to reduce this fundam ...
The need to visualize molecular structure in the course of a chemical reaction, a phase transformation or a biological function has been a dream of scientists for decades. The development of time-resolved X-ray and electron-based methods is making this tru ...
A review. Time-resolved X-ray absorption fine structure (XAFS) spectroscopy with picosecond temporal resoln. is a new method to observe electronic and geometric structures of short-lived reaction intermediates. It combines an intense femtosecond laser sour ...
The advanced characteristics of synchrotron light has led in recent years to the development of a series of new experimental techniques to investigate chemical and physical properties on a microscopic scale. Although originally developed for materials scie ...
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Recently, much attention has been devoted to the development of new pulsed sources of radiation for investigating matter with atomic scale temporal and spatial resolution. While much has been achieved thanks to modern ultrafast laser technology, the ultima ...
