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Asymmetric Total Synthesis of (-)-Arborisidine and (-)-19-epi-Arborisidine Enabled by a Catalytic Enantioselective Pictet-Spengler Reaction

Publications associées (32)

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Bright solitons in non-equilibrium coherent quantum matter

Hugo Pierre Alexandre Flayac

We theoretically demonstrate a mechanism for bright soliton generation in spinor non-equilibrium Bose-Einstein condensates made of atoms or quasi-particles such as polaritons in semiconductor microcavities. We give analytical expressions for bright (half) ...

Royal Soc2016

Accelerated path integral methods for atomistic simulations at ultra-low temperatures

Michele Ceriotti, Felix Uhl

Path integral methods provide a rigorous and systematically convergent framework to include the quantum mechanical nature of atomic nuclei in the evaluation of the equilibrium properties of molecules, liquids, or solids at finite temperature. Such nuclear ...

American Institute of Physics2016

Quantum antiferromagnets have proven to be some of the cleanest realizations available for theoretical, numerical, and experimental studies of quantum fluctuation effects. At finite temperatures, however, the additional effects of thermal fluctuations in t ...

2016

Condensation phase diagram of cavity polaritons in GaN-based microcavities: Experiment and theory

Nicolas Grandjean, Jean-François Carlin, Raphaël Butté, Eric Feltin, Jacques Levrat

The evolution of the polariton condensation threshold (P-thr) under incoherent optical pumping is investigated both theoretically and experimentally over a wide range of temperatures (4-340 K) and exciton-cavity photon detunings (-120-0 meV) in a multiple ...

2010

We report a room-temperature measurement of nanomechanical motion with an imprecision below the standard quantum limit (SQL), using cavity-enhanced optical near fields. Fundamental thermodynamical cavity frequency fluctuation limits the total imprecision t ...

2010

Quantum confinement dependence of the energy splitting and recombination dynamics of A and B excitons in a GaN/AlGaN quantum well

Nicolas Grandjean, Jean-François Carlin, Raphaël Butté, Eric Feltin, Dobri Simeonov, Massimo Gurioli

We report the observation of well-resolved A and B excitonic resonances in the reflectivity spectra of a wedged GaN/AlGaN quantum well (QW) with 5% Al content in the barriers for different well thicknesses. For the thicker well cases, the energy splitting ...

2009

Phase diagram of a polariton laser from cryogenic to room temperature

Nicolas Grandjean, Jean-François Carlin, Raphaël Butté, Eric Feltin, Jacques Levrat, Gabriel Christmann

The signature of the strong-coupling regime is unambiguously evidenced in a GaN-based microcavity (MC) above the polariton lasing threshold P-thr at room temperature through the observation of the upper polariton branch. The MC system exhibits a renormaliz ...

2009

Fast temperature cycling of the catalytic CO oxidation using microstructure reactors

Martin Luther

The possibility to increase the performance (productivity or selectivity) of a chemical reactor by using periodic variations of reaction parameters (e.g. reactant concentration or temperature) has been theoretically envisaged since the beginning of the 70t ...

EPFL2008

Introductory Thermodynamics

Pierre Infelta

The fundamental aspects of classical thermodynamics are presented in a simple compact way. The equations derived are illustrated by numerous (111) examples, often direct application of the relations just obtained. The (four) laws of thermodynamics are pres ...

Overseas Press India Private Limited2006

A model Ni-Bi system has been used to investigate intergranular penetration (IGP) phenomenon. All experiments have been done on Ni 26° bicrystal at 700°C using bismuth vapour condensation as a source of liquid bismuth. Such a procedure results at room ...

2005