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Robust Interfacial Modifier for Efficient Perovskite Solar Cells: Reconstruction of Energy Alignment at Buried Interface by Self-Diffusion of Dopants

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Molecularly Engineered Hole Transporting Materials for High Performance Perovskite Solar Cells

Kasparas Rakstys

Perovskite solar cells have rapidly revolutionized the photovoltaic research showing an im-pressively dynamic progress on power conversion efficiency from 3.8 to 22% in only several years, a record for a nascent technology. Furthermore, inexpensive precurs ...

EPFL2018

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Li-TFSI is the most common p-dopant for the hole conductor spiro-MeOTAD in the normal structure (n-i-p) of perovskite solar cells (PSCs), which consistently yield the highest power conversion efficiency (PCE) albeit at the risk of lower long-term operation ...

ROYAL SOC CHEMISTRY2018

In this work, we analyze the carrier recombination kinetics and the associated charge carrier density in methylammonium lead iodide perovskite (MAPI) solar cells that use mesoporous TiO2, as selective contact (m-MAPI) and flat solar cells (without the meso ...

Amer Chemical Soc2017

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Hole transport matertial (HTM) as charge selective layer in perovskite solar cells (PSCs) plays an important role in achieving high power conversion efficiency (PCE). It is known that the dopants and additives are necessary in the HTM in order to improve t ...

Wiley-V C H Verlag Gmbh2017

Undoubtedly, perovskite solar cells have become a key player in 3rd generation photovoltaics over the last few years. Although it is only in 2012 that the first solid state perovskite solar cell was reported, power conversion efficiencies have increased so ...

EPFL2017

Charge Collection in Hybrid Perovskite Solar Cells: Relation to the Nanoscale Elemental Distribution

Christophe Ballif, Björn Niesen, Michael Elias Stückelberger, Jérémie Werner

Unveiling the correlation between elemental composition, Fermi-level splitting, and charge collection in perovskite solar cells (PSCs) when exposed to different environments is crucial to understanding the origin of defects. This will enable defect enginee ...

Ieee-Inst Electrical Electronics Engineers Inc2017

Microscopic Analysis of Inherent Void Passivation in Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Yonghui Lee

The presence of voids in perovskite solar cells influences the efficiency because of accelerated charge recombination. The induced electric field near voids due to band bending attracts photogenerated electrons and holes toward the voids, leading to carrie ...

Amer Chemical Soc2017

We report the presence of defects in CH3NH3PbI3, which is one of the main factors that deteriorates the performance of perovskite solar cells. Although the efficiency of the perovskite solar cells has been improved by curing defects using various methods, ...

Royal Soc Chemistry2017

Inorganic p-Type Semiconductors: Their Applications and Progress in Dye-Sensitized Solar Cells and Perovskite Solar Cells

Jun Ho Yum, Soo-Jin Moon, Peter Chen, Meng Li

Considering the increasing global demand for energy and the harmful ecological impact of conventional energy sources, it is obvious that development of clean and renewable energy is a necessity. Since the Sun is our only external energy source, harnessing ...

MDPI2016

Dopant-Free Donor (D)--D--D Conjugated Hole-Transport Materials for Efficient and Stable Perovskite Solar Cells

Shaik Mohammed Zakeeruddin, Jingshan Luo, Chenyi Yi, Dongqin Bi, Xiong Li, Fei Zhang, Shilong Wang

Three novel hole-transporting materials (HTMs) using the 4-methoxytriphenylamine (MeOTPA) core were designed and synthesized. The energy levels of the HTMs were tuned to match the perovskite energy levels by introducing symmetrical electron-donating groups ...

Wiley-VCH Verlag Berlin2016